Highly fluorescent, water-soluble, size-tunable gold quantum dots

被引:1017
作者
Zheng, J [1 ]
Zhang, CW [1 ]
Dickson, RM [1 ]
机构
[1] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA
基金
美国国家卫生研究院; 美国国家科学基金会;
关键词
D O I
10.1103/PhysRevLett.93.077402
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Highly fluorescent, water-soluble, few-atom Au quantum dots have been created that behave as multielectron artificial atoms with discrete, size-tunable electronic transitions throughout the visible and near IR. Correlation of nanodot sizes with emission energies fits the simple relation, E-Fermi/N-1/3, predicted by the jellium model. Providing the "missing link" between atomic and nanoparticle behavior in noble metals, these emissive, water-soluble Au nanoclusters open new opportunities for biological labels, energy transfer pairs, and light emitting sources in nanoscale optoelectronics.
引用
收藏
页码:077402 / 1
页数:4
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