Air-sea CO2 fluxes on the US Middle Atlantic Bight

被引:91
作者
DeGrandpre, MD
Olbu, GJ
Beatty, CM
Hammar, TR
机构
[1] Univ Montana, Dept Chem, Missoula, MT 59812 USA
[2] Woods Hole Oceanog Inst, Dept Appl Phys & Engn, Woods Hole, MA 02543 USA
基金
美国国家科学基金会;
关键词
D O I
10.1016/S0967-0645(02)00122-4
中图分类号
P7 [海洋学];
学科分类号
0707 ;
摘要
One objective of the Ocean Margins Program (OMP) was to quantify air-sea CO2 fluxes on the US Middle Atlantic Bight (MAB). No measurements of the partial pressure of CO2 (pCO(2)) had been reported for the MAB prior to the 1994 OMP field program. A number of field studies have now taken place that include ship and mooring-based measurements Of pCO(2) spanning the years 1994-2000. We use these data to quantify the annual air-sea CO2, flux on the MAB. These calculations indicate that the MAB is a net annual sink for atmospheric CO2, with the inner, mid, and outer-shelf regions taking up similar to0.1, 0.7, and 0.2 Mt C yr(-1), respectively, for a net uptake of similar to 1+/-0.6 Mt C yr(-1). The annual cycle of heating and cooling combined with high winds during the period of undersaturation (winter) appear to account for a significant portion of the uptake. The flux uncertainty is dominated by uncertainty of the gas-transfer velocity parameterization, atmospheric CO2 levels, and coarse spatial pCO(2) resolution. Errors due to monthly averaging of wind and pCO(2) time-series are relatively small in comparison. Recent results from other ocean margin regions found a significantly larger flux (in mol m(-2)yr(-1)). Unlike the MAB, the increase in pCO(2) due to summer heating appears to be counterbalanced by new production and the pCO(2) never rises significantly above atmospheric saturation in these areas. (C) 2002 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:4355 / 4367
页数:13
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