Modeling of potential power plant plume impacts on Dallas-Fort Worth visibility

被引:4
作者
Seigneur, C
Pai, P
Tombach, I
McDade, C
Saxena, P
Mueller, P
机构
[1] Atmospher & Environm Res Inc, San Ramon, CA 94583 USA
[2] ENSR Corp, Camarillo, CA 93012 USA
[3] Elect Power Res Inst, Environm Div, Palo Alto, CA 94304 USA
来源
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION | 2000年 / 50卷 / 05期
关键词
D O I
10.1080/10473289.2000.10464121
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
During wintertime, haze episodes occur in the Dallas-Ft. Worth (DFW) urban area. Such episodes are characterized by substantial light scattering by particles and relatively low absorption, leading to so-called "white haze." The objective of this work was to assess whether reductions in the emissions of SO2 from specific coal-fired power plants located over 100 km from DFW could lead to a discernible change in the DFW white haze. To that end, the transport, dispersion, deposition, and chemistry of the plume of a major power plant were simulated using a reactive plume model (ROME). The realism of the plume model simulations was tested by comparing model calculations of plume concentrations with aircraft data of SF6 tracer concentrations and ozone concentrations. A second-order closure dispersion algorithm was shown to perform better than a first-order closure algorithm and the empirical Pasquill-Gifford-Turner algorithm. For plume impact assessment, three actual scenarios were simulated, two With clear-sky conditions and one with the presence of fog prior to the haze. The largest amount of sulfate formation was obtained for the fog episode. Therefore, a hypothetical scenario was constructed using the meteorological conditions of the fog episode with input data values adjusted to be more conducive to sulfate formation. The results of the simulations suggest that reductions in the power plant emissions lead to less than proportional reductions in sulfate concentrations in DFW for the fog scenario. Calculations of the associated effects on light scattering using Mie theory suggest that reduction in total (plume + ambient) light extinction of less than 13% would be obtained with a 44% reduction in emissions of SO2 from the modeled power plant.
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页码:835 / 848
页数:14
相关论文
共 24 条
[1]   KINETICS AND MECHANISM OF THE FORMATION OF HYDROXYMETHANESULFONIC ACID AT LOW PH [J].
BOYCE, SD ;
HOFFMANN, MR .
JOURNAL OF PHYSICAL CHEMISTRY, 1984, 88 (20) :4740-4746
[2]  
*ENSR, 1990, 3750002010 ENSR CONS
[3]   Evaluation of the reactive and optics model of emissions (ROME) [J].
Gabruk, RS ;
Sykes, RI ;
Seigneur, C ;
Pai, P ;
Gillespie, P ;
Bergstrom, RW ;
Saxena, P .
ATMOSPHERIC ENVIRONMENT, 1999, 33 (03) :383-399
[4]  
Hoffman M. R., 1985, CHEM TRANSFORMATION, VII
[5]   Reduced gas phase kinetic mechanisms for atmospheric plume chemistry [J].
Karamchandani, P ;
Koo, A ;
Seigneur, C .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1998, 32 (11) :1709-1720
[6]   ATMOSPHERIC GAS-AEROSOL EQUILIBRIUM .3. THERMODYNAMICS OF CRUSTAL ELEMENTS CA2+, K+, AND MG2+ [J].
KIM, YP ;
SEINFELD, JH .
AEROSOL SCIENCE AND TECHNOLOGY, 1995, 22 (01) :93-110
[7]   ATMOSPHERIC GAS-AEROSOL EQUILIBRIUM .2. ANALYSIS OF COMMON APPROXIMATIONS AND ACTIVITY-COEFFICIENT CALCULATION METHODS [J].
KIM, YP ;
SEINFELD, JH ;
SAXENA, P .
AEROSOL SCIENCE AND TECHNOLOGY, 1993, 19 (02) :182-198
[8]   ATMOSPHERIC GAS AEROSOL EQUILIBRIUM .1. THERMODYNAMIC MODEL [J].
KIM, YP ;
SEINFELD, JH ;
SAXENA, P .
AEROSOL SCIENCE AND TECHNOLOGY, 1993, 19 (02) :157-181
[9]  
LOWENTHAL D, 1994, DOCUMENTATION MANUAL
[10]  
LOWENTHAL D, 1996, COMMUNICATION