Development of the electronic structure in a K-doped C-60 monolayer on a Ag(111) surface

被引:100
作者
Tjeng, LH
Hesper, R
Heessels, ACL
Heeres, A
Jonkman, HT
Sawatzky, GA
机构
[1] Solid State Physics Laboratory, Materials Science Centre, University of Groningen, 9747 AG Groningen
关键词
fullerenes; surfaces and interfaces; photoelectron spectroscopies;
D O I
10.1016/S0038-1098(97)00126-9
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
We present an electron spectroscopy study of the development of the electronic structure in the K-doped C-60 monolayer on a Ag(1 1 1) surface. We find that the occupation of the lowest unoccupied molecular orbital (LUMO) of the C-60 can be varied continuously from 0.75 (undoped) to 6.0 (fully doped). We also find that the density of states at the Fermi level for a doping level corresponding to 3 electrons per C-60 is at least a factor of two higher than that found from photoemission on bulk K3C60. This enhanced density of states at the Fermi level might suggest an increased superconducting transition temperature for the monolayer system. (C) 1997 Elsevier Science Ltd.
引用
收藏
页码:31 / 35
页数:5
相关论文
共 37 条
[21]   SATELLITES IN THE PHOTOEMISSION SPECTRA OF A3C60 (A = K AND RB) [J].
KNUPFER, M ;
MERKEL, M ;
GOLDEN, MS ;
FINK, J ;
GUNNARSSON, O ;
ANTROPOV, VP .
PHYSICAL REVIEW B, 1993, 47 (20) :13944-13947
[22]   STRESSED C-60 LAYERS ON AU(001) [J].
KUK, Y ;
KIM, DK ;
SUH, YD ;
PARK, KH ;
NOH, HP ;
OH, SJ ;
KIM, SK .
PHYSICAL REVIEW LETTERS, 1993, 70 (13) :1948-1951
[23]   BAND-GAP, EXCITONS AND COULOMB INTERACTIONS OF SOLID C-60 [J].
LOF, RW ;
VANVEENENDAAL, MA ;
JONKMAN, HT ;
SAWATZKY, GA .
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 1995, 72 :83-87
[24]   BAND-GAP, EXCITONS, AND COULOMB INTERACTION IN SOLID C-60 [J].
LOF, RW ;
VANVEENENDAAL, MA ;
KOOPMANS, B ;
JONKMAN, HT ;
SAWATZKY, GA .
PHYSICAL REVIEW LETTERS, 1992, 68 (26) :3924-3927
[25]   ELECTRONIC-STRUCTURES OF C-60 AND C-70 ADSORBED ON THE CU(111) SURFACE AND INTRAMOLECULAR STM IMAGES [J].
MARUYAMA, Y ;
OHNO, K ;
KAWAZOE, Y .
PHYSICAL REVIEW B, 1995, 52 (03) :2070-2075
[26]   PHOTOEMISSION, AUTOIONIZATION, AND X-RAY-ABSORPTION SPECTROSCOPY OF ULTRATHIN-FILM C60 ON AU(110) [J].
MAXWELL, AJ ;
BRUHWILER, PA ;
NILSSON, A ;
MARTENSSON, N ;
RUDOLF, P .
PHYSICAL REVIEW B, 1994, 49 (15) :10717-10725
[27]   C-60 ON AL(111) - COVALENT BONDING AND SURFACE RECONSTRUCTION [J].
MAXWELL, AJ ;
BRUHWILER, PA ;
ANDERSSON, S ;
ARVANITIS, D ;
HERNNAS, B ;
KARIS, O ;
MANCINI, DC ;
MARTENSSON, N ;
GRAY, SM ;
JOHANSSON, MKJ ;
JOHANSSON, LSO .
PHYSICAL REVIEW B, 1995, 52 (08) :R5546-R5549
[28]   PHOTOEMISSION-STUDY OF THE ELECTRONIC-STRUCTURE OF C-60 AND KXC-60 [J].
MERKEL, M ;
KNUPFER, M ;
GOLDEN, MS ;
FINK, J ;
SEEMANN, R ;
JOHNSON, RL .
PHYSICAL REVIEW B, 1993, 47 (17) :11470-11478
[29]   DETERMINATION OF CHARGE STATES OF C-60 ADSORBED ON METAL-SURFACES [J].
MODESTI, S ;
CERASARI, S ;
RUDOLF, P .
PHYSICAL REVIEW LETTERS, 1993, 71 (15) :2469-2472
[30]   ELECTRONIC-STRUCTURE OF KXC-60 STUDIED BY HIGH-ENERGY RESOLVED PHOTOEMISSION SPECTROSCOPY [J].
MORIKAWA, T ;
TAKAHASHI, T .
SOLID STATE COMMUNICATIONS, 1993, 87 (11) :1017-1021