High-Performance Non-Fullerene Polymer Solar Cells Based on a Pair of Donor-Acceptor Materials with Complementary Absorption Properties

被引:234
作者
Lin, Haoran [1 ,2 ,3 ]
Chen, Shangshang [1 ,2 ,3 ]
Li, Zhengke [1 ,2 ,3 ]
Lai, Joshua Yuk Lin [2 ,3 ]
Yang, Guofang [2 ,3 ]
McAfee, Terry [4 ,5 ]
Jiang, Kui [2 ,3 ]
Li, Yunke [2 ,3 ]
Liu, Yuhang [2 ,3 ]
Hu, Huawei [2 ,3 ]
Zhao, Jingbo [2 ,3 ]
Ma, Wei [6 ]
Ade, Harald [4 ,5 ]
Yan, He [1 ,2 ,3 ]
机构
[1] Hong Kong Univ Sci & Technol, Shenzhen Res Inst, Shenzhen 518057, Peoples R China
[2] Hong Kong Univ Sci & Technol, Dept Chem, Clear Water Bay, Hong Kong, Peoples R China
[3] Hong Kong Univ Sci & Technol, Energy Inst, Clear Water Bay, Hong Kong, Peoples R China
[4] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA
[5] N Carolina State Univ, Organ & Carbon Elect Lab, Raleigh, NC 27695 USA
[6] Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China
基金
美国国家科学基金会;
关键词
OPEN-CIRCUIT VOLTAGE; ELECTRON-ACCEPTOR; HIGH-EFFICIENCY; SMALL-MOLECULE; 3D STRUCTURE; MORPHOLOGY; COPOLYMERS; FLUORINE; RECOMBINATION; AGGREGATION;
D O I
10.1002/adma.201502775
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A 7.3% efficiency non-fullerene polymer solar cell is realized by combining a large-bandgap polymer PffT2-FTAZ-2DT with a small-bandgap acceptor IEIC. The complementary absorption of donor polymer and small-molecule acceptor is responsible for the high-performance of the solar-cell device. This work provides important guidance to improve the performance of non-fullerene polymer solar cells.
引用
收藏
页码:7299 / +
页数:7
相关论文
共 52 条
[21]   Dramatic performance enhancement for large bandgap thick-film polymer solar cells introduced by a difluorinated donor unit [J].
Li, Zhengke ;
Lin, Haoran ;
Jiang, Kui ;
Carpenter, Joshua ;
Li, Yunke ;
Liu, Yuhang ;
Hu, Huawei ;
Zhao, Jingbo ;
Ma, Wei ;
Ade, Harald ;
Yan, He .
NANO ENERGY, 2015, 15 :607-615
[22]   High-performance fullerene-free polymer solar cells with 6.31% efficiency [J].
Lin, Yuze ;
Zhang, Zhi-Guo ;
Bai, Huitao ;
Wang, Jiayu ;
Yao, Yuehan ;
Li, Yongfang ;
Zhu, Daoben ;
Zhan, Xiaowei .
ENERGY & ENVIRONMENTAL SCIENCE, 2015, 8 (02) :610-616
[23]   An Electron Acceptor Challenging Fullerenes for Efficient Polymer Solar Cells [J].
Lin, Yuze ;
Wang, Jiayu ;
Zhang, Zhi-Guo ;
Bai, Huitao ;
Li, Yongfang ;
Zhu, Daoben ;
Zhan, Xiaowei .
ADVANCED MATERIALS, 2015, 27 (07) :1170-1174
[24]   Non-fullerene acceptors for organic photovoltaics: an emerging horizon [J].
Lin, Yuze ;
Zhan, Xiaowei .
MATERIALS HORIZONS, 2014, 1 (05) :470-488
[25]   A star-shaped electron acceptor based on 5,5′-bibenzothiadiazole for solution processed solar cells [J].
Lin, Yuze ;
Wang, Haifeng ;
Li, Yongfang ;
Zhu, Daoben ;
Zhan, Xiaowei .
JOURNAL OF MATERIALS CHEMISTRY A, 2013, 1 (46) :14627-14632
[26]   A Solution-Processable Electron Acceptor Based on Dibenzosilole and Diketopyrrolopyrrole for Organic Solar Cells [J].
Lin, Yuze ;
Li, Yongfang ;
Zhan, Xiaowei .
ADVANCED ENERGY MATERIALS, 2013, 3 (06) :724-728
[27]   A 3D star-shaped non-fullerene acceptor for solution-processed organic solar cells with a high open-circuit voltage of 1.18 V [J].
Lin, Yuze ;
Cheng, Pei ;
Li, Yongfang ;
Zhan, Xiaowei .
CHEMICAL COMMUNICATIONS, 2012, 48 (39) :4773-4775
[28]   Effect of Fluorine Content in Thienothiophene-Benzodithiophene Copolymers on the Morphology and Performance of Polymer Solar Cells [J].
Liu, Peng ;
Zhang, Kai ;
Liu, Feng ;
Jin, Yaocheng ;
Liu, Shengjian ;
Russell, Thomas P. ;
Yip, Hin-Lap ;
Huang, Fei ;
Cao, Yong .
CHEMISTRY OF MATERIALS, 2014, 26 (09) :3009-3017
[29]   D-A copolymers based on 5,6-difluorobenzotriazole and oligothiophenes: Synthesis, field effect transistors, and polymer solar cells [J].
Liu, Xuncheng ;
Cai, Ping ;
Chen, Zhenhui ;
Zhang, Lianjie ;
Zhang, Xiaofei ;
Sun, Jiangman ;
Wang, Haitao ;
Chen, Junwu ;
Peng, Junbiao ;
Chen, Hongzheng ;
Cao, Yong .
POLYMER, 2014, 55 (07) :1707-1715
[30]   A Tetraphenylethylene Core-Based 3D Structure Small Molecular Acceptor Enabling Efficient Non-Fullerene Organic Solar Cells [J].
Liu, Yuhang ;
Mu, Cheng ;
Jiang, Kui ;
Zhao, Jingbo ;
Li, Yunke ;
Zhang, Lu ;
Li, Zhengke ;
Lai, Joshua Yuk Lin ;
Hu, Huawei ;
Ma, Tingxuan ;
Hu, Rongrong ;
Yu, Demei ;
Huang, Xuhui ;
Tang, Ben Zhong ;
Yan, He .
ADVANCED MATERIALS, 2015, 27 (06) :1015-1020