The observation of a surface resonance state in the valence-band structure of the perovskite La0.65Ba0.35MnO3

被引:16
作者
Waldfried, C [1 ]
McIlroy, DN [1 ]
Liou, SH [1 ]
Sabiryanov, R [1 ]
Jaswal, SS [1 ]
Dowben, PA [1 ]
机构
[1] UNIV NEBRASKA,CTR MAT RES & ANAL,LINCOLN,NE 68588
关键词
D O I
10.1088/0953-8984/9/5/009
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The valence-band electronic structure of a crystalline thin film of La0.65Ba0.35MnO3 has been investigated using angle-resolved photoemission. The observed valence-band structure has a substantial surface contribution and is strongly influenced by the surface conditions. Surface contamination and disorder attenuate the emission from a Mn-3d-derived state at a binding energy of 3.3 eV. This state was found to bt localized at the surface with dispersion only in the plane of the surface and exhibited a strong intensity dependence on emission angle. On the basis of a simple LMTO-ASA bulk band calculation, it is clear that this state does not fall within a bulk band gap. We have therefore identified this Mn-3d-derived state at 3.3 eV below E(F) as a surface resonance.
引用
收藏
页码:1031 / 1038
页数:8
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