Direct observation of mixed-parity excited states in surface-passivated PbS nanocrystals

被引:8
作者
Fernée, MJ [1 ]
Watt, A
Warner, J
Heckenberg, N
Rubinsztein-Dunlop, H
机构
[1] Univ Queensland, Ctr Quantum Comp Technol, Dept Phys, Brisbane, Qld 4072, Australia
[2] Univ Queensland, Ctr Biophoton & Laser Sci, Dept Phys, Brisbane, Qld 4072, Australia
关键词
D O I
10.1088/0957-4484/15/9/040
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Photoluminescent emission is observed from surface-passivated PbS nanocrystals following the two-photon excitation of high-energy excitonic states. The emission appears directly at the excitation energy with no detectable Stokes-shift for a wide range of excitation energies. The observation of direct emission from states excited by two-photon absorption indicates that the parity of the excited states of surface-passivated PbS nanocrystals is partially mixed.
引用
收藏
页码:1351 / 1355
页数:5
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