Photocurrent generation in random networks of multiwall-carbon-nanotubes grown by an "all-laser" process

被引:28
作者
El Khakani, M. A. [1 ]
Le Borgne, V. [1 ]
Aissa, B. [1 ]
Rosei, F. [1 ]
Scilletta, C. [2 ]
Speiser, E. [2 ]
Scarselli, M. [2 ]
Castrucci, P. [2 ]
De Crescenzi, M. [2 ]
机构
[1] INRS Energie Mat & Telecommun, Inst Natl Rech Sci, Varennes, PQ J3X 1S2, Canada
[2] Univ Roma Tor Vergata, Dept Fis, Unita CNISM, I-00133 Rome, Italy
关键词
carbon nanotubes; laser materials processing; nanofabrication; photoconductivity; photovoltaic effects; Schottky barriers;
D O I
10.1063/1.3211958
中图分类号
O59 [应用物理学];
学科分类号
摘要
We report photocurrent generation in entangled networks of multiwall-carbon nanotubes (MWCNTs) grown on TiN/Si substrates by an all-laser process. By integrating these MWCNTs into planar devices, we demonstrate that they generate photocurrent over all the visible and near-ultraviolet range, with maximum efficiency around 420 nm. Photocurrent is obtained even at zero applied voltage, pointing to a true photovoltaic (PV) effect. The extracted photocurrent as a function of applied voltage exhibits nonlinear behavior for voltages >= 2 V, suggesting that the devices do not behave as pure photoresistances. Other mechanisms (e.g., Schottky barriers imbalance) are invoked to describe current flow in these PV devices.
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页数:3
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