Giant Rabi splitting between localized mixed plasmon-exciton states in a two-dimensional array of nanosize metallic disks in an organic semiconductor

被引:122
作者
Bellessa, J. [1 ,2 ,3 ,6 ]
Symonds, C. [1 ,2 ,3 ]
Vynck, K. [6 ]
Lemaitre, A. [7 ]
Brioude, A. [1 ,4 ,5 ]
Beaur, L. [6 ]
Plenet, J. C. [1 ,2 ,3 ]
Viste, P. [1 ,2 ,3 ]
Felbacq, D. [6 ]
Cambril, E. [7 ]
Valvin, P. [6 ]
机构
[1] Univ Lyon, F-69622 Villeurbanne, France
[2] Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France
[3] CNRS, UMR 5586, F-69622 Villeurbanne, France
[4] Univ Lyon 1, LMI, F-69622 Villeurbanne, France
[5] CNRS, UMR 5615, F-69622 Villeurbanne, France
[6] Univ Montpellier 2, CNRS, GES, F-34095 Montpellier 5, France
[7] CNRS, LPN, F-91460 Marcoussis, France
关键词
D O I
10.1103/PhysRevB.80.033303
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We study localized surface plasmons in strong coupling with excitons of organic semiconductors. The plasmons are localized in lithographed silver nanodisks organized in square array. A giant Rabi splitting energy of 450 meV is obtained, and typical behaviors of mixed states, i.e., anticrossing of their energies and crossing of their linewidths, are observed. Three-dimensional finite-difference time-domain simulations and coupled oscillator calculations are used to analyze and corroborate the experimental results.
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页数:4
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