Comparison of air pollutant emissions among mega-cities

被引:119
作者
Parrish, David D. [1 ]
Kuster, William C. [1 ]
Shao, Min [2 ]
Yokouchi, Yoko [3 ]
Kondo, Yutaka [4 ]
Goldan, Paul D. [1 ]
de Gouw, Joost A. [1 ,5 ]
Koike, Makoto [6 ]
Shirai, Tomoko [7 ]
机构
[1] NOAA, Earth Syst Res Lab, Div Chem Sci, Boulder, CO 80305 USA
[2] Peking Univ, Coll Environm Sci & Engn, Beijing 100871, Peoples R China
[3] Natl Inst Environm Studies, Div Environm Chem, Tsukuba, Ibaraki, Japan
[4] Univ Tokyo, Adv Sci & Technol Res Ctr, Tokyo, Japan
[5] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
[6] Univ Tokyo, Grad Sch Sci, Dept Earth & Planetary Sci, Tokyo 113, Japan
[7] Natl Inst Environm Studies, Ctr Global Environm Res, Tsukuba, Ibaraki, Japan
关键词
Mega-city; Emissions; Carbon monoxide; Nitrogen oxides; NOx; Hydrocarbons; VOC; HYDROCARBONS;
D O I
10.1016/j.atmosenv.2009.06.024
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Ambient measurements of hydrocarbons, carbon monoxide and nitrogen oxides from three mega-cities (Beijing, Mexico City, Tokyo) are compared with similar measurements from US cities in the mid-1980s and the early 2000s. The common hydrocarbon pattern seen in all data sets suggests that emissions associated with gasoline-fueled vehicles dominate in all of these cities. This commonality suggests that it will be efficient and, ultimately, cost effective to proceed with vehicular emission controls in most emerging mega-cities, while proceeding with development of more locally appropriate air quality control strategies through emissions inventory development and ambient air monitoring. Over the three decades covered by the US data sets, the hydrocarbon emissions decreased by a significant factor (something like an order of magnitude), which is greater than suggested by emission inventories, particularly the EDGAR international inventory. The ambient hydrocarbon and CO concentrations reported for the three non-US mega-cities are higher than present US ambient concentrations. but lower than those observed in the 1980s in the US. The one exception to the preceding statement is the high concentrations of CO observed in Beijing, which apparently have a large regional contribution. Published by Elsevier Ltd.
引用
收藏
页码:6435 / 6441
页数:7
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