Confined optical phonon modes in aligned nanorod arrays detected by resonant inelastic light scattering

被引:40
作者
Nobile, Concetta
Fonoberov, Vladimir A.
Kudera, Stefan
Della Torre, Antonio
Ruffino, Antonio
Chilla, Gerwin
Kipp, Tobias
Heitmann, Detlef
Manna, Liberato
Cingolani, Roberto
Balandin, Alexander A.
Krahne, Roman
机构
[1] CNR, INFM, Natl Nanotechnol Lab, I-73100 Lecce, Italy
[2] Univ Calif Riverside, Dept Elect Engn, Riverside, CA 92521 USA
[3] Univ Hamburg, Inst Appl Phys, D-20355 Hamburg, Germany
关键词
D O I
10.1021/nl062818+
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We investigated the optical phonon excitations of laterally aligned nanorod arrays by resonant Raman scattering. We observed a strong suppression of the surface-optical phonon modes in the closely packed aligned arrays and a small asymmetry in the longitudinal-optical phonon peak with respect to the rod alignment orientation. These observations can be explained by the spatial distribution of the potential of the different phonon modes derived from the first principles calculations.
引用
收藏
页码:476 / 479
页数:4
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共 31 条
[1]   Electrical control of Forster energy transfer [J].
Becker, Klaus ;
Lupton, John M. ;
Mueller, Josef ;
Rogach, Andrey L. ;
Talapin, Dmitri V. ;
Weller, Horst ;
Feldmann, Jochen .
NATURE MATERIALS, 2006, 5 (10) :777-781
[2]   THEORY OF ONE-PHONON RAMAN-SCATTERING IN SEMICONDUCTOR MICROCRYSTALLITES [J].
CHAMBERLAIN, MP ;
TRALLEROGINER, C ;
CARDONA, M .
PHYSICAL REVIEW B, 1995, 51 (03) :1680-1693
[3]   Interface and confined optical phonons in wurtzite nanocrystals [J].
Fonoberov, VA ;
Balandin, AA .
PHYSICAL REVIEW B, 2004, 70 (23) :1-4
[4]   Polar optical phonons in wurtzite spheroidal quantum dots: theory and application to ZnO and ZnO/MgZnO nanostructures [J].
Fonoberov, VA ;
Balandin, AA .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2005, 17 (07) :1085-1097
[5]   ZnO quantum dots: Physical properties and optoelectronic applications [J].
Fonoberov, Vladimir A. ;
Balandin, Alexander A. .
JOURNAL OF NANOELECTRONICS AND OPTOELECTRONICS, 2006, 1 (01) :19-38
[6]   Self-assembled stripe patterns of CdS nanorods [J].
Ghezelbash, Ali ;
Koo, Bonil ;
Korgel, Brian A. .
NANO LETTERS, 2006, 6 (08) :1832-1836
[7]   Electroluminescence from a single-nanocrystal transistor [J].
Gudiksen, MS ;
Maher, KN ;
Ouyang, L ;
Park, H .
NANO LETTERS, 2005, 5 (11) :2257-2261
[8]   Surface optical phonions in gallium phosphide nanowires [J].
Gupta, R ;
Xiong, Q ;
Mahan, GD ;
Eklund, PC .
NANO LETTERS, 2003, 3 (12) :1745-1750
[9]   Rectifying behavior of electrically aligned ZnO nanorods [J].
Harnack, O ;
Pacholski, C ;
Weller, H ;
Yasuda, A ;
Wessels, JM .
NANO LETTERS, 2003, 3 (08) :1097-1101
[10]   Linearly polarized emission from colloidal semiconductor quantum rods [J].
Hu, JT ;
Li, LS ;
Yang, WD ;
Manna, L ;
Wang, LW ;
Alivisatos, AP .
SCIENCE, 2001, 292 (5524) :2060-2063