Electron dynamics and level broadening in slow atomic interactions with metal surfaces and thin metallic films

被引:13
作者
Bahrim, B
Kürpick, P
Thumm, U
Wille, U
机构
[1] Hahn Meitner Inst Berlin GmbH, Bereich Theoret Phys, D-14109 Berlin, Germany
[2] Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA
[3] Harvard Smithsonian Ctr Astrophys, Inst Theoret Atom & Mol Phys, Cambridge, MA 02138 USA
基金
美国国家科学基金会;
关键词
D O I
10.1016/S0168-583X(99)01158-1
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
Theoretical results on the electron dynamics and on resonant level broadening in slow atomic interactions with metal surfaces and thin metallic films are presented. Within the time-dependent close-coupling method, a wave-packet approach is introduced in which nondiagonal couplings in the subspace of metal states are taken into account. This approach is applied in a study of the time evolution of the occupation of hydrogen states in front of a semi-infinite metal. First-order level widths are calculated for hydrogenic atoms interacting with thin metallic Alms. They are found to exhibit pronounced size-quantization effects arising from the confinement of the electronic motion in the growth direction of the film. (C) 2000 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:614 / 625
页数:12
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