REVEAL: Characterizing fine aerosols in the Fraser Valley, BC

被引:12
作者
Pryor, SC
Barthelmie, RJ
Hoff, RM
Sakiyama, S
Simpson, R
Steyn, D
机构
[1] RISO NATL LAB,DEPT METEOROL & WIND ENGN,ROSKILDE,DENMARK
[2] MINIST ENVIRONM LANDS & PARKS,VICTORIA,BC,CANADA
[3] GRIFFITH UNIV,FAC ENVIRONM SCI,NATHAN,QLD 4111,AUSTRALIA
[4] UNIV BRITISH COLUMBIA,DEPT GEOG,VANCOUVER,BC V5Z 1M9,CANADA
基金
加拿大自然科学与工程研究理事会;
关键词
D O I
10.1080/07055900.1997.9649592
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
The REVEAL field study was conducted during July and August 1993 to document the chemical and physical characteristics of ambient fine aerosols in southwestern British Columbia (B.C.) (particularly the Lower. Fraser Valley (LFV)) and to quantify the impact of those aerosols upon visibility in the LFV A description of the study motivations, objectives and monitoring protocols are presented herein along with results of analyses conducted using the REVEAL datasets. It is shown that: visibility and aerosol concentrations/composition are highly variable in. the temporal and spatial dimensions, and while organic matter dominates fine aerosol mass (accounting for 35-46% of the mean fine aerosol mass) in the LFV, nitrate this region. The severity of visibility impairment in the valley despite comparatively low fine and sulphate dominate particle light scattering (b(SP)) (accounting for 55-67% of mean b(SP)) in mass concentrations is attributed to the high mass scattering efficiencies of the ambient aerosols (due in part to the relative abundance of ammonia/ium). Source types of ambient fine aerosols at four of the monitoring sites are identified using Principal Components Analysis (PCA), and used to calculate first approximations of mass contributions by source type using repression analysis. Results indicate that direct vehicle emissions, secondary aerosols and soil/road dust dominate the sources of fine aerosols in the LFV. Analysis of supplementary data indicates that the REVEAL monitoring period was characterized by fairly typical summertime visibility and meteorological conditions for the region and hence that it is possible to generalize from these analyses. The gross spatial features of the secondary fine aerosol distribution in the LFV are explained in relation to the prevailing meteorology and spatial patterns of precursor emissions.
引用
收藏
页码:209 / 227
页数:19
相关论文
共 28 条
[1]  
BARTHELMIE RJ, 1996, P 89 ANN A WMA C JUN
[2]   ATMOSPHERIC EQUILIBRIUM-MODEL OF SULFATE AND NITRATE AEROSOLS [J].
BASSETT, M ;
SEINFELD, JH .
ATMOSPHERIC ENVIRONMENT, 1983, 17 (11) :2237-2252
[3]   ANTHROPOGENIC NH3 EMISSIONS IN EUROPE [J].
BUIJSMAN, E ;
MAAS, HFM ;
ASMAN, WAH .
ATMOSPHERIC ENVIRONMENT, 1987, 21 (05) :1009-1022
[4]  
ELDRED RA, 1990, IMPROVE NPS NETWORKS, P187
[5]  
Finlayson-Pitts B.J., 1986, Atmospheric Chemistry: Fundamentals and Experimental Techniques
[6]  
GUISEBAGLEY L, 1994, AEROSOLS ATMOSPHERIC, P429
[7]  
*GVRD, 1994, GVRD AIR QUAL MAN PL
[8]   DEVELOPMENT AND TESTING OF A NEW VARIABLE SCALE AIR-POLLUTION MODEL - ACDEP [J].
HERTEL, O ;
CHRISTENSEN, J ;
RUNGE, EH ;
ASMAN, WAH ;
BERKOWICZ, R ;
HOVMAND, MF ;
HOV, O .
ATMOSPHERIC ENVIRONMENT, 1995, 29 (11) :1267-1290
[9]  
Horvath H., 1992, ATMOSPHERIC ACIDITY
[10]   MEASUREMENTS OF CONCENTRATIONS AND DRY SURFACE FLUXES OF ATMOSPHERIC NITRATES IN THE PRESENCE OF AMMONIA [J].
HUEBERT, BJ ;
LUKE, WT ;
DELANY, AC ;
BROST, RA .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1988, 93 (D6) :7127-7136