Effect of Groundwater Iron and Phosphate on the Efficacy of Arsenic Removal by Iron-Amended BioSand Filters

被引:86
作者
Chiew, Hannah [1 ]
Sampson, M. L. [1 ]
Huch, Sokhan [1 ]
Ken, Sreymom [1 ]
Bostick, Benjamin C. [2 ]
机构
[1] RDI C Resource Dev Int Cambodia, Kean Svay, Kandal, Cambodia
[2] Dartmouth Coll, Dept Earth Sci, Hanover, NH 03755 USA
关键词
ZERO-VALENT IRON; ZEROVALENT IRON; DRINKING-WATER; CAMBODIA; SAND; BANGLADESH; SILICATE; VIETNAM; NITRATE; MEKONG;
D O I
10.1021/es803444t
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Naturally occurring arsenic in groundwater in Cambodia is a serious health concern, This study tested the efficacy of a BioSand filter amended with iron nails, Kanchan filter, as a household water treatment option with three natural arsenic-bearing groundwater sources of varying compositions and spiked with lab cultured E. coli and MS2. The effectiveness of arsenic and pathogen removal was not constant over time and was highly dependent on the influent composition, The filter was relatively ineffective intreating arsenic contaminated groundwater and effluent arsenic concentrations were between 74 and 226 mu g L-1, which is higher than accepted drinking water standards. The overall average arsenic removal was 39.4, 74.9, and 45.4%, respectively, and the extent of arsenic removal was riot related to the influent arsenic concentration. The main reasons for poor arsenic removal was due to the combination of high influent P (>0.5 mg L-1) and low Fe (<5 mg L-1) concentrations and that the added iron nails were largely ineffective due to insufficient contact time with the water. The findings suggest that such amended filters should not be widely deployed until improvements are made to address the consistency and efficacy of treatment. In addition, the filter poses some potential health risk associated with the production of elevated nitrate levels in the effluent within the filter, possibly due to nitrification and high levels of ammonia in the groundwater.
引用
收藏
页码:6295 / 6300
页数:6
相关论文
共 33 条
[31]   Occurrence of nitrification in chloraminated distribution systems [J].
Wilczak, A ;
Jacangelo, JG ;
Marcinko, JP ;
Odell, LH ;
Kirmeyer, GJ ;
Wolfe, RL .
JOURNAL AMERICAN WATER WORKS ASSOCIATION, 1996, 88 (07) :74-85
[32]  
Zhang H, 2003, AQUATIC ARSENIC TOXICITY AND TREATMENT, P19
[33]  
2007, GUIDELINES PREPARATI