Enhanced third-order nonlinear optical properties of C60-silane compounds

被引:20
作者
Yu, BL [1 ]
Xia, HP [1 ]
Zhu, CS [1 ]
Gan, FX [1 ]
机构
[1] Chinese Acad Sci, Shanghai Inst Opt & Fine Mech, Shanghai 201800, Peoples R China
基金
中国国家自然科学基金;
关键词
D O I
10.1063/1.1512959
中图分类号
O59 [应用物理学];
学科分类号
摘要
The nonlinear optical properties of C-60[NH2-(CH2)(3)-Si(OC2H5)(3)](3) sol and gel were investigated by femtosecond optical Kerr gate technique at 820 nm. The nonresonant third-order optical susceptibilities were measured to be 1.4x10(-13) and 1.6x10(-13) esu for the C-60[NH2-(CH2)(3)-Si(OC2H5)(3)](3) sol and gel, respectively, which are two orders larger than that of C-60 molecule. (C) 2002 American Institute of Physics.
引用
收藏
页码:2701 / 2703
页数:3
相关论文
共 17 条
[1]   NONLINEAR OPTICAL-GLASSES FOR ULTRAFAST OPTICAL SWITCHES [J].
FRIBERG, SR ;
SMITH, PW .
IEEE JOURNAL OF QUANTUM ELECTRONICS, 1987, 23 (12) :2089-2094
[2]   Measurement of the resonant third-order nonlinear susceptibility of C-60 by nondegenerate four-wave mixing [J].
Geng, L ;
Wright, JC .
CHEMICAL PHYSICS LETTERS, 1996, 249 (1-2) :105-111
[3]   NONRESONANT 3RD-ORDER OPTICAL NONLINEARITY OF ALL-CARBON MOLECULES C-60 [J].
GONG, QH ;
SUN, YX ;
XIA, ZJ ;
ZOU, YH ;
GU, ZN ;
ZHOU, XH ;
DI, Q .
JOURNAL OF APPLIED PHYSICS, 1992, 71 (06) :3025-3026
[4]  
KADISH KM, 1994, RECENT ADV CHEM PHYS, P92
[5]   Universal exciton size scaling in π conjugated systems [J].
Knupfer, M ;
Fink, J ;
Zojer, E ;
Leising, G ;
Fichou, D .
CHEMICAL PHYSICS LETTERS, 2000, 318 (06) :585-589
[6]   Wavelength dependence of photoreduction of Ag+ ions in glasses through the multiphoton process [J].
Kondo, Y ;
Inouye, H ;
Fujiwara, S ;
Suzuki, T ;
Mitsuyu, T ;
Yoko, T ;
Hirao, K .
JOURNAL OF APPLIED PHYSICS, 2000, 88 (03) :1244-1250
[7]   Measurement of the second-order molecular hyperpolarizability of fullerene anions by CARS spectroscopy [J].
Lascola, R ;
Wright, JC .
CHEMICAL PHYSICS LETTERS, 1998, 290 (1-3) :117-124
[8]   Femtosecond third-order optical nonlinearity of C60 and its derivative at a wavelength of 810 nm [J].
Li, JL ;
Wang, SF ;
Yang, H ;
Gong, QH ;
An, X ;
Chen, HY ;
Qiang, D .
CHEMICAL PHYSICS LETTERS, 1998, 288 (2-4) :175-178
[9]   FEMTOSECOND TIME-RESOLVED INTERFEROMETRY FOR THE DETERMINATION OF COMPLEX NONLINEAR SUSCEPTIBILITY [J].
MINOSHIMA, K ;
TAIJI, M ;
KOBAYASHI, T .
OPTICS LETTERS, 1991, 16 (21) :1683-1685
[10]   Size scaling of third-order off-resonant polarizabilities. Electronic coherence in organic oligomers [J].
Schulz, M ;
Tretiak, S ;
Chernyak, V ;
Mukamel, S .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2000, 122 (03) :452-459