Development of ferromagnetism in the doped topological insulator Bi2-xMnxTe3

被引:414
作者
Hor, Y. S. [1 ]
Roushan, P. [2 ]
Beidenkopf, H. [2 ]
Seo, J. [2 ]
Qu, D. [2 ]
Checkelsky, J. G. [2 ]
Wray, L. A. [2 ]
Hsieh, D. [2 ]
Xia, Y. [2 ]
Xu, S. -Y. [2 ]
Qian, D. [2 ]
Hasan, M. Z. [2 ]
Ong, N. P. [2 ]
Yazdani, A. [2 ]
Cava, R. J. [1 ]
机构
[1] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA
[2] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA
基金
美国国家科学基金会;
关键词
PHYSICS;
D O I
10.1103/PhysRevB.81.195203
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The development of ferromagnetism in Mn-doped Bi2Te3 is characterized through measurements on a series of single crystals with different Mn content. Scanning tunneling microscopy analysis shows that the Mn substitutes on the Bi sites, forming compounds of the type Bi2-xMnxTe3, and that the Mn substitutions are randomly distributed, not clustered. Mn doping first gives rise to local magnetic moments with Curie-like behavior, but by the compositions Bi1.96Mn0.04Te3 and Bi1.91Mn0.09Te3, a second-order ferromagnetic transition is observed, with T(C similar to)9-12 K. The easy axis of magnetization in the ferromagnetic phase is perpendicular to the Bi2Te3 basal plane. Thermoelectric power and Hall effect measurements show that the Mn-doped Bi2Te3 crystals are p-type. Angle-resolved photoemission spectroscopy measurements show that the topological surface states that are present in pristine Bi2Te3 are also present at 15 K in ferromagnetic Mn-doped Bi2-xMnxTe3 and that the dispersion relations of the surface states are changed in a subtle fashion.
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页数:7
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