Nonlinear wavepacket interferometry for polyatomic molecules

被引:38
作者
Cina, JA [1 ]
机构
[1] Univ Oregon, Dept Chem, Eugene, OR 97403 USA
[2] Univ Oregon, Oregon Ctr Opt, Eugene, OR 97403 USA
关键词
D O I
10.1063/1.1319873
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We investigate the application of a previously considered nonlinear wavepacket interferometry scheme to molecules with a single stable conformation in the electronic ground state. It is shown that interference experiments with pairs of phase-locked ultrashort pulse-pairs can be used to determine the complex overlaps of a nonstationary nuclear wavefunction evolving in an excited electronic state with a collection of compact displaced wavepackets moving in specified ways in the ground-state potential. (C) 2000 American Institute of Physics. [S0021-9606(00)00145-8].
引用
收藏
页码:9488 / 9496
页数:9
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