High-performing submicron organic thin-film transistors fabricated by residue-free embossing

被引:30
作者
Auner, Christoph [1 ]
Palfinger, Ursula [1 ]
Gold, Herbert [1 ]
Kraxner, Johanna [1 ]
Haase, Anja [1 ]
Haber, Thomas [2 ]
Sezen, Meltem [2 ]
Grogger, Werner [2 ]
Jakopic, Georg [1 ]
Krenn, Joachim R. [1 ]
Leising, G. [3 ]
Stadlober, Barbara [1 ]
机构
[1] Joanneum Res GmbH, Inst Nanostructured Mat & Photon, A-8160 Weiz, Austria
[2] Graz Univ Technol, Inst Electron Microscopy, A-8010 Graz, Austria
[3] Graz Univ Technol, Inst Solid State Phys, A-8010 Graz, Austria
关键词
Organic thin-film transistors; Nanoimprint lithography; Hot Embossing; Submicron channel length; FIELD-EFFECT TRANSISTORS; NM CHANNEL-LENGTH; ROLL-TO-ROLL; NANOIMPRINT LITHOGRAPHY; LOW-VOLTAGE;
D O I
10.1016/j.orgel.2009.12.012
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
In this study, we report on an innovative residue-free nanoimprint lithography process for the patterning of submicron-spaced contacts, used as source and drain electrodes in down-scaled organic thin-film transistors. The method is based on thermally initiated radical polymerization of a novel imprint resist whose outstanding chemical and physical properties are responsible for the excellent results in processability and structure transfer. In combination with a pretreated stamp the thermally curable resist enables residue-free imprinting, thus making etching obsolete. In addition, this process implies only moderate temperature budgets and it is eco-friendly due to a water-based lift-off. To validate the process, source and drain patterned submicron organic thin-film transistors with pentacene as the semiconductor were fabricated, which show excellent transistor behavior parameterized by a low switch-on voltage of V-so = -3 V, an on-off ratio of more than 10(5) and a charge carrier mobility of mu = 0.25 cm(2)/V s. (C) 2009 Elsevier B. V. All rights reserved.
引用
收藏
页码:552 / 557
页数:6
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