Detection and characterization of longitudinal field for tip-enhanced Raman spectroscopy

被引:229
作者
Hayazawa, N [1 ]
Saito, Y
Kawata, S
机构
[1] RIKEN, Nanophoton Lab, Wako, Saitama 3510198, Japan
[2] Japan Corp Sci & Technol, CREST, Tokyo, Japan
[3] Osaka Univ, Dept Appl Phys, Osaka 5650871, Japan
关键词
D O I
10.1063/1.1839646
中图分类号
O59 [应用物理学];
学科分类号
摘要
We characterized the longitudinal field formed at a tightly focused spot by a high numerical aperture objective lens using a tip-enhanced near-field microscope. The longitudinal field efficiently excites the localized surface plasmon polaritons at the metallic tip apex resulting in an electric field enhancement. Radially polarized light generated by a combination of four half-waveplates successfully increases the longitudinal field resulting in higher sensitivity for tip-enhanced Raman spectroscopy of adenine nanocrystals. (C) 2004 American Institute of Physics.
引用
收藏
页码:6239 / 6241
页数:3
相关论文
共 21 条
[1]   Locally enhanced Raman spectroscopy with an atomic force microscope [J].
Anderson, MS .
APPLIED PHYSICS LETTERS, 2000, 76 (21) :3130-3132
[2]   Near-field scattering of longitudinal fields [J].
Bouhelier, A ;
Beversluis, MR ;
Novotny, L .
APPLIED PHYSICS LETTERS, 2003, 82 (25) :4596-4598
[3]   Near-field second-harmonic generation induced by local field enhancement [J].
Bouhelier, A ;
Beversluis, M ;
Hartschuh, A ;
Novotny, L .
PHYSICAL REVIEW LETTERS, 2003, 90 (01) :4
[4]   Sharper focus for a radially polarized light beam [J].
Dorn, R ;
Quabis, S ;
Leuchs, G .
PHYSICAL REVIEW LETTERS, 2003, 91 (23)
[5]   Local field enhancement with an apertureless near-field-microscope probe [J].
Furukawa, H ;
Kawata, S .
OPTICS COMMUNICATIONS, 1998, 148 (4-6) :221-224
[6]   High-resolution near-field Raman microscopy of single-walled carbon nanotubes -: art. no. 095503 [J].
Hartschuh, A ;
Sánchez, EJ ;
Xie, XS ;
Novotny, L .
PHYSICAL REVIEW LETTERS, 2003, 90 (09) :4
[7]  
Hayazawa N, 1999, J MICROSC-OXFORD, V194, P472, DOI 10.1046/j.1365-2818.1999.00563.x
[8]   Metallized tip amplification of near-field Raman scattering [J].
Hayazawa, N ;
Inouye, Y ;
Sekkat, Z ;
Kawata, S .
OPTICS COMMUNICATIONS, 2000, 183 (1-4) :333-336
[9]   Detection of an individual single-wall carbon nanotube by tip-enhanced near-field Raman spectroscopy [J].
Hayazawa, N ;
Yano, T ;
Watanabe, H ;
Inouye, Y ;
Kawata, S .
CHEMICAL PHYSICS LETTERS, 2003, 376 (1-2) :174-180
[10]   Near-field Raman scattering enhanced by a metallized tip [J].
Hayazawa, N ;
Inouye, Y ;
Sekkat, Z ;
Kawata, S .
CHEMICAL PHYSICS LETTERS, 2001, 335 (5-6) :369-374