A Facile One-step Method to Produce Graphene-CdS Quantum Dot Nanocomposites as Promising Optoelectronic Materials

被引:675
作者
Cao, Aoneng [1 ]
Liu, Zhen [1 ]
Chu, Saisai [2 ]
Wu, Minghong [1 ]
Ye, Zhangmei [1 ]
Cai, Zhengwei [1 ]
Chang, Yanli [1 ]
Wang, Shufeng [2 ]
Gong, Qihuang [2 ]
Liu, Yuanfang [1 ,3 ]
机构
[1] Shanghai Univ, Inst Nanochem & Nanobiol, Shanghai 200444, Peoples R China
[2] Peking Univ, State Key Lab Mesoscop Phys, Sch Phys, Beijing 100871, Peoples R China
[3] Peking Univ, Beijing Natl Lab Mol Sci, Coll Chem & Mol Engn, Beijing 100871, Peoples R China
关键词
EXFOLIATED GRAPHITE OXIDE; AQUEOUS DISPERSIONS; REDUCTION; SHEETS; ASSEMBLIES;
D O I
10.1002/adma.200901920
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A single-layer graphene-CdS quantum dot nanocomposite is synthesized by a one-step reaction from graphene oxide, and thus avoids the low-yield production and the aggregation of single-layer graphene sheets. This new graphene-based material shows promising optoelectronic properties. Picosecond ultrafast electron transfer from the US quantum dots to the graphene sheets has been observed by time-resolved fluorescence spectroscopy.
引用
收藏
页码:103 / +
页数:5
相关论文
共 27 条
[1]   Synthesis and characterization of carbon nanotube-nanocrystal heterostructures [J].
Banerjee, S ;
Wong, SS .
NANO LETTERS, 2002, 2 (03) :195-200
[2]   Electronic confinement and coherence in patterned epitaxial graphene [J].
Berger, Claire ;
Song, Zhimin ;
Li, Xuebin ;
Wu, Xiaosong ;
Brown, Nate ;
Naud, Cecile ;
Mayou, Didier ;
Li, Tianbo ;
Hass, Joanna ;
Marchenkov, Atexei N. ;
Conrad, Edward H. ;
First, Phillip N. ;
de Heer, Wait A. .
SCIENCE, 2006, 312 (5777) :1191-1196
[3]   Rashba effect in the graphene/Ni(111) system [J].
Dedkov, Yu. S. ;
Fonin, M. ;
Ruediger, U. ;
Laubschat, C. .
PHYSICAL REVIEW LETTERS, 2008, 100 (10)
[4]   Deoxygenation of Exfoliated Graphite Oxide under Alkaline Conditions: A Green Route to Graphene Preparation [J].
Fan, Xiaobin ;
Peng, Wenchao ;
Li, Yang ;
Li, Xianyu ;
Wang, Shulan ;
Zhang, Guoliang ;
Zhang, Fengbao .
ADVANCED MATERIALS, 2008, 20 (23) :4490-4493
[5]   The rise of graphene [J].
Geim, A. K. ;
Novoselov, K. S. .
NATURE MATERIALS, 2007, 6 (03) :183-191
[6]   Electronic transport properties of individual chemically reduced graphene oxide sheets [J].
Gomez-Navarro, Cristina ;
Weitz, R. Thomas ;
Bittner, Alexander M. ;
Scolari, Matteo ;
Mews, Alf ;
Burghard, Marko ;
Kern, Klaus .
NANO LETTERS, 2007, 7 (11) :3499-3503
[7]   Electrochemical assembly of a CdS semiconductor nanoparticle monolayer on surfaces: Structural properties and photoelectrochemical applications [J].
Granot, E ;
Patolsky, F ;
Willner, I .
JOURNAL OF PHYSICAL CHEMISTRY B, 2004, 108 (19) :5875-5881
[8]   High-yield production of graphene by liquid-phase exfoliation of graphite [J].
Hernandez, Yenny ;
Nicolosi, Valeria ;
Lotya, Mustafa ;
Blighe, Fiona M. ;
Sun, Zhenyu ;
De, Sukanta ;
McGovern, I. T. ;
Holland, Brendan ;
Byrne, Michele ;
Gun'ko, Yurii K. ;
Boland, John J. ;
Niraj, Peter ;
Duesberg, Georg ;
Krishnamurthy, Satheesh ;
Goodhue, Robbie ;
Hutchison, John ;
Scardaci, Vittorio ;
Ferrari, Andrea C. ;
Coleman, Jonathan N. .
NATURE NANOTECHNOLOGY, 2008, 3 (09) :563-568
[9]   Synthesis and characterization of CdS/multiwalled carbon nanotube heterojunctions [J].
Huang, Q ;
Gao, L .
NANOTECHNOLOGY, 2004, 15 (12) :1855-1860
[10]   PREPARATION OF GRAPHITIC OXIDE [J].
HUMMERS, WS ;
OFFEMAN, RE .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1958, 80 (06) :1339-1339