Strong exciton-photon coupling and exciton hybridization in a thermally evaporated polycrystalline film of an organic small molecule

被引：136

作者：

Holmes, RJ ^{[1
]}

Forrest, SR ^{[1
]}

机构：

[1] Princeton Univ, Dept Elect Engn, Princeton Inst Sci & Technol Mat, Princeton, NJ 08544 USA

来源：

PHYSICAL REVIEW LETTERS | 2004年 / 93卷 / 18期

关键词：

D O I：

10.1103/PhysRevLett.93.186404

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We demonstrate strong exciton-photon coupling in an optical microcavity containing a thermally evaporated polycrystalline organic thin film. Microcavity polaritons result from coupling between the 0-0 excitonic transition of 3,4,7,8 napthalenetetracarboxylic dianhydride and a cavity photon. For thicker films, the 0-1 transition also couples to the cavity mode, as vibronic relaxation is overcome by the short Rabi period for strong coupling. To our knowledge, this is the first report of strong coupling between a cavity photon and multiple vibronic transitions in a single material, made possible by the pronounced vibronic absorption features characteristic of crystalline organic materials.

引用

页码：186404 / 1

页数：4

共 18 条

[1] Cavity polaritons in microcavities containing disordered organic semiconductors [J].

Agranovich, VM ;

Litinskaia, M ;

Lidzey, DG .

PHYSICAL REVIEW B, 2003, 67 (08)

[2] Polariton-induced optical asymmetry in semiconductor microcavities [J].

Armitage, A ;

Skolnick, MS ;

Kavokin, AV ;

Whittaker, DM ;

Astratov, VN ;

Gehring, GA ;

Roberts, JS .

PHYSICAL REVIEW B, 1998, 58 (23) :15367-15370

[3] ORGANIC-ON-INORGANIC SEMICONDUCTOR CONTACT BARRIER DIODES .2. DEPENDENCE ON ORGANIC FILM AND METAL CONTACT PROPERTIES [J].

FORREST, SR ;

KAPLAN, ML ;

SCHMIDT, PH .

JOURNAL OF APPLIED PHYSICS, 1984, 56 (02) :543-551

[4] Ultrathin organic films grown by organic molecular beam deposition and related techniques [J].

Forrest, SR .

CHEMICAL REVIEWS, 1997, 97 (06) :1793-1896

[5] Tunable polariton absorption of distributed feedback microcavities at room temperature [J].

Fujita, T ;

Sato, Y ;

Kuitani, T ;

Ishihara, T .

PHYSICAL REVIEW B, 1998, 57 (19) :12428-12434

[6] MEASUREMENT OF CAVITY-POLARITON DISPERSION CURVE FROM ANGLE-RESOLVED PHOTOLUMINESCENCE EXPERIMENTS [J].

HOUDRE, R ;

WEISBUCH, C ;

STANLEY, RP ;

OESTERLE, U ;

PELLANDINI, P ;

ILEGEMS, M .

PHYSICAL REVIEW LETTERS, 1994, 73 (15) :2043-2046

[7] Strong exciton-photon coupling in an organic semiconductor microcavity [J].

Lidzey, DG ;

Bradley, DDC ;

Skolnick, MS ;

Virgili, T ;

Walker, S ;

Whittaker, DM .

NATURE, 1998, 395 (6697) :53-55

[8] Photon-mediated hybridization of Frenkel excitons in organic semiconductor microcavities [J].

Lidzey, DG ;

Bradley, DDC ;

Armitage, A ;

Walker, S ;

Skolnick, MS .

SCIENCE, 2000, 288 (5471) :1620-1623

[9] Room temperature polariton emission from strongly coupled organic semiconductor microcavities [J].

Lidzey, DG ;

Bradley, DDC ;

Virgili, T ;

Armitage, A ;

Skolnick, MS ;

Walker, S .

PHYSICAL REVIEW LETTERS, 1999, 82 (16) :3316-3319

[10] High-temperature ultrafast polariton parametric amplification in semiconductor microcavities [J].

Saba, M ;

Ciuti, C ;

Bloch, J ;

Thierry-Mieg, V ;

André, R ;

Dang, LS ;

Kundermann, S ;

Mura, A ;

Bongiovanni, G ;

Staehli, JL ;

Deveaud, B .

NATURE, 2001, 414 (6865) :731-735

← 1 2 →