Enhanced haze pollution by black carbon in megacities in China

被引:676
作者
Ding, A. J. [1 ,2 ,3 ]
Huang, X. [1 ,2 ,3 ]
Nie, W. [1 ,2 ,3 ]
Sun, J. N. [1 ,2 ,3 ]
Kerminen, V. -M. [4 ]
Petaja, T. [2 ,4 ]
Su, H. [1 ,2 ,3 ,5 ]
Cheng, Y. F. [5 ]
Yang, X. -Q. [1 ,3 ]
Wang, M. H. [1 ,2 ,3 ]
Chi, X. G. [1 ,2 ,3 ]
Wang, J. P. [1 ,3 ]
Virkkula, A. [1 ,2 ,4 ,6 ]
Guo, W. D. [1 ,2 ,3 ]
Yuan, J. [1 ,3 ]
Wang, S. Y. [1 ,2 ,3 ]
Zhang, R. J. [2 ,7 ]
Wu, Y. F. [2 ,7 ]
Song, Y. [8 ]
Zhu, T. [2 ,8 ]
Zilitinkevich, S. [4 ,6 ]
Kulmala, M. [4 ]
Fu, C. B. [1 ,2 ,3 ]
机构
[1] Nanjing Univ, Sch Atmospher Sci, Inst Climate & Global Change Res, Nanjing 210008, Jiangsu, Peoples R China
[2] Joint Int Res Lab Atmospher & Earth Syst Sci, Nanjing, Jiangsu, Peoples R China
[3] Collaborat Innovat Ctr Climate Change, Nanjing, Jiangsu, Peoples R China
[4] Univ Helsinki, Dept Phys, Helsinki, Finland
[5] Max Planck Inst Chem, Multiphase Chem Dept, Mainz, Germany
[6] Finnish Meteorol Inst, FIN-00101 Helsinki, Finland
[7] Chinese Acad Sci, Inst Atmospher Phys, Key Lab Climate Environm Temerate East Asia, Beijing, Peoples R China
[8] Peking Univ, Coll Environm Sci & Engn, Beijing 100871, Peoples R China
基金
芬兰科学院;
关键词
planetary boundary layer; feedback; radiative forcing; air pollution; SYNOPTIC WEATHER; EASTERN CHINA; AIR-POLLUTION; MIXING STATE; JANUARY; 2013; AEROSOLS; IMPACT; EVENTS; LAYER;
D O I
10.1002/2016GL067745
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
Aerosol-planetary boundary layer (PBL) interactions have been found to enhance air pollution in megacities in China. We show that black carbon (BC) aerosols play the key role in modifying the PBL meteorology and hence enhancing the haze pollution. With model simulations and data analysis from various field observations in December 2013, we demonstrate that BC induces heating in the PBL, particularly in the upper PBL, and the resulting decreased surface heat flux substantially depresses the development of PBL and consequently enhances the occurrences of extreme haze pollution episodes. We define this process as the dome effect of BC and suggest an urgent need for reducing BC emissions as an efficient way to mitigate the extreme haze pollution in megacities of China.
引用
收藏
页码:2873 / 2879
页数:7
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