Optical spectroscopy of two-dimensional layered (C6H5C2H4-NH3)2-PbI4 perovskite

被引:254
作者
Gauthron, K. [1 ]
Lauret, J-S. [2 ]
Doyennette, L. [2 ]
Lanty, G. [2 ]
Al Choueiry, A. [2 ]
Zhang, S. J. [2 ]
Brehier, A. [2 ]
Largeau, L. [1 ]
Mauguin, O. [1 ]
Bloch, J. [1 ]
Deleporte, E. [2 ]
机构
[1] CNRS, Lab Photon & Nanostruct, F-91460 Marcoussis, France
[2] Ecole Normale Super, Lab Photon Quant & Mol, F-94235 Cachan, France
来源
OPTICS EXPRESS | 2010年 / 18卷 / 06期
关键词
QUANTUM-WELL STRUCTURES; SEMICONDUCTOR; EXCITONS; (C10H21NH3)2PBI4; TEMPERATURE; ELECTROLUMINESCENCE; (C6H13NH3)(2)PBI4; COMPOUND; PBI2;
D O I
10.1364/OE.18.005912
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We report on optical spectroscopy (photoluminescence and photoluminescence excitation) on two-dimensional self-organized layers of (C6H5C2H4-NH3)(2)-PbI4 perovskite. Temperature and excitation power dependance of the optical spectra gives a new insight into the excitonic and the phononic properties of this hybrid organic/inorganic semiconductor. In particular, exciton-phonon interaction is found to be more than one order of magnitude higher than in GaAs QWs. As a result, photoluminescence emission lines have to be interpreted in the framework of a polaron model. (C) 2010 Optical Society of America
引用
收藏
页码:5912 / 5919
页数:8
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