Three-dimensional imaging of colloidal glasses under steady shear

被引:214
作者
Besseling, R.
Weeks, Eric R.
Schofield, A. B.
Poon, W. C. K.
机构
[1] Univ Edinburgh, Scottish Univ Phys Alliance, Edinburgh EH9 3JZ, Midlothian, Scotland
[2] Univ Edinburgh, Sch Phys, Edinburgh EH9 3JZ, Midlothian, Scotland
[3] Emory Univ, Dept Phys, Atlanta, GA 30322 USA
基金
英国工程与自然科学研究理事会;
关键词
HIGHLY SUPERCOOLED LIQUIDS; HARD-SPHERE SUSPENSIONS; SELF-DIFFUSION; DIRECT VISUALIZATION; INDUCED ORDER; FLOW; DYNAMICS; MICROSCOPY; SOFT; HETEROGENEITIES;
D O I
10.1103/PhysRevLett.99.028301
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Using fast confocal microscopy we image the three-dimensional dynamics of particles in a yielded hard-sphere colloidal glass under steady shear. The structural relaxation, observed in regions with uniform shear, is nearly isotropic but is distinctly different from that of quiescent metastable colloidal fluids. The inverse relaxation time tau(-1)(alpha) and diffusion constant D, as functions of the local shear rate (gamma) over dot, show marked shear thinning with tau(-1)(alpha)proportional to D proportional to (gamma) over dot(0.8) over more than two decades in (gamma) over dot. In contrast, the global rheology of the system displays Herschel-Bulkley behavior. We discuss the possible role of large scale shear localization and other mechanisms in generating this difference.
引用
收藏
页数:4
相关论文
共 45 条
  • [1] SHEAR-INDUCED ORDER IN SUSPENSIONS OF HARD-SPHERES
    ACKERSON, BJ
    PUSEY, PN
    [J]. PHYSICAL REVIEW LETTERS, 1988, 61 (08) : 1033 - 1036
  • [2] Shear profiles and localization in simulations of granular materials
    Aharonov, Einat
    Sparks, David
    [J]. Physical Review E - Statistical, Nonlinear, and Soft Matter Physics, 2002, 65 (05): : 1 - 051302
  • [3] Yielding and flow in adhesive and nonadhesive concentrated emulsions
    Bécu, L
    Manneville, S
    Colin, A
    [J]. PHYSICAL REVIEW LETTERS, 2006, 96 (13)
  • [4] Yield stress, heterogeneities and activated processes in soft glassy materials
    Berthier, L
    [J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 2003, 15 (11) : S933 - S943
  • [5] Nonequilibrium dynamics and fluctuation-dissipation relation in a sheared fluid
    Berthier, L
    Barrat, JL
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2002, 116 (14) : 6228 - 6242
  • [6] Laponite: Aging and shear rejuvenation of a colloidal glass
    Bonn, D
    Tanase, S
    Abou, B
    Tanaka, H
    Meunier, J
    [J]. PHYSICAL REVIEW LETTERS, 2002, 89 (01) : 157011 - 157014
  • [7] Measurement of the full shear-induced self-diffusion tensor of noncolloidal suspensions
    Breedveld, V
    van den Ende, D
    Bosscher, M
    Jongschaap, RJJ
    Mellema, J
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2002, 116 (23) : 10529 - 10535
  • [8] Shear-induced configurations of confined colloidal suspensions
    Cohen, I
    Mason, TG
    Weitz, DA
    [J]. PHYSICAL REVIEW LETTERS, 2004, 93 (04) : 046001 - 1
  • [9] Slip, yield, and bands in colloidal crystals under oscillatory shear
    Cohen, Itai
    Davidovitch, Benny
    Schofield, Andrew B.
    Brenner, Michael P.
    Weitz, David A.
    [J]. PHYSICAL REVIEW LETTERS, 2006, 97 (21)
  • [10] Direct visualization of ageing in colloidal glasses
    Courtland, RE
    Weeks, ER
    [J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 2003, 15 (01) : S359 - S365