Photochemical ozone formation in north west Europe and its control

被引：210

作者：

Derwent, RG ^{[1
]}

Jenkin, ME

Saunders, SM

Pilling, MJ

Simmonds, PG

Passant, NR

Dollard, GJ

Dumitrean, P

Kent, A

机构：

[1] Meteorol Off, Climate Res, Bracknell RG12 2SZ, Berks, England

[2] Univ London Imperial Coll Sci Technol & Med, Dept Environm Sci & Technol, Ascot RG12 2SZ, Berks, England

[3] Univ Western Australia, Sch Earth & Geog Sci, Crawley, WA, Australia

[4] Univ Leeds, Sch Chem, Leeds RG12 2SZ, W Yorkshire, England

[5] Univ Bristol, Sch Chem, Bristol RG12 2SZ, Avon, England

[6] AEA Technol, NETCEN, Culham, Oxon, England

来源：

ATMOSPHERIC ENVIRONMENT | 2003年 / 37卷 / 14期

基金：

英国自然环境研究理事会;

关键词：

ozone; motor vehicle emissions; UN ECE VOC protocol; chemical mechanism; organic compounds in urban areas;

D O I：

10.1016/S1352-2310(03)00031-1

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

A photochemical trajectory model together with a Master Chemical Mechanism and a highly speciated emission inventory for organic compounds have been used to describe the formation of ozone in north west Europe and to identify the most prolific ozone-forming organic compounds. Observations are reviewed to assess the impact of emission controls on their urban volatile organic compound (VOC) concentration trends with time. The observed trends are then used to deduce the likely trends in episodic peak ozone concentrations and to compare them with observed trends in peak ozone concentrations. It is concluded that it is likely that motor vehicle emission controls have brought about a substantial reduction in episodic peak ozone concentrations in north west Europe during the 1990s. (C) 2003 Elsevier Science Ltd. All rights reserved.

引用

页码：1983 / 1991

页数：9

共 14 条

[1] APPLICATION OF SENSITIVITY AND UNCERTAINTY ANALYSIS TECHNIQUES TO A PHOTOCHEMICAL OZONE MODEL [J].

DERWENT, R ;

HOV, O .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1988, 93 (D5) :5185-5199

[2] Photochemical ozone creation potentials for organic compounds in northwest Europe calculated with a master chemical mechanism [J].

Derwent, RG ;

Jenkin, ME ;

Saunders, SM ;

Pilling, MJ .

ATMOSPHERIC ENVIRONMENT, 1998, 32 (14-15) :2429-2441

[3] Analysis and interpretation of the continuous hourly monitoring data for 26 C2-C8 hydrocarbons at 12 United Kingdom sites during 1996 [J].

Derwent, RG ;

Davies, TJ ;

Delaney, M ;

Dollard, GJ ;

Field, RA ;

Dumitrean, P ;

Nason, PD ;

Jones, BMR ;

Pepler, SA .

ATMOSPHERIC ENVIRONMENT, 2000, 34 (02) :297-312

[4]

DOLLARD GJ, 1995, ISSUES ENV SCI TECHN, V4, P37

[5]

*EMEP, 2001, 12001 EMEP DNMI

[6] Protocol for the development of the Master Chemical Mechanism, MCM v3 (Part B): tropospheric degradation of aromatic volatile organic compounds [J].

Jenkin, ME ;

Saunders, SM ;

Wagner, V ;

Pilling, MJ .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2003, 3 :181-193

[7] The tropospheric degradation of volatile organic compounds: A protocol for mechanism development [J].

Jenkin, ME ;

Saunders, SM ;

Pilling, MJ .

ATMOSPHERIC ENVIRONMENT, 1997, 31 (01) :81-104

[8]

*NORD COUNC MIN, 1991, PHOT OX ATMS NORD

[9]

Passant N. R., 2002, SPECIATION UK EMISSI

[10] Protocol for the development of the Master Chemical Mechanism, MCM v3 (Part A): tropospheric degradation of non-aromatic volatile organic compounds [J].

Saunders, SM ;

Jenkin, ME ;

Derwent, RG ;

Pilling, MJ .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2003, 3 :161-180

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