Engineering directed excitonic energy transfer

被引：28

作者：

Perdomo, Alejandro ^{[1
]}

Vogt, Leslie ^{[1
]}

Najmaie, Ali ^{[1
]}

Aspuru-Guzik, Alan ^{[1
]}

机构：

[1] Harvard Univ, Dept Chem & Biol Chem, Cambridge, MA 02138 USA

来源：

APPLIED PHYSICS LETTERS | 2010年 / 96卷 / 09期

基金：

加拿大自然科学与工程研究理事会;

关键词：

excitons; nanostructured materials; quantum dots; DYNAMICS; SYSTEMS; COMPLEXES; PHOTOSYNTHESIS; RELAXATION; COHERENCE;

D O I：

10.1063/1.3323108

中图分类号：

O59 [应用物理学];

学科分类号：

摘要：

We provide an intuitive platform for engineering exciton transfer dynamics. We show that careful consideration of the spectral density, which describes the system-bath interaction, leads to opportunities to engineer exciton transfer. Since excitons in nanostructures are proposed for use in quantum information processing and artificial photosynthetic designs, our approach paves the way for engineering a wide range of desired exciton dynamics. We carefully describe the validity of the model and use experimentally relevant material parameters to show counter-intuitive examples of directed exciton transfer in a linear chain of quantum dots.

引用

页数：3

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