Spatially Selective Optical Tuning of Quantum Dot Thin Film Luminescence

被引:20
作者
Chen, Jixin [1 ]
Chan, Yang-Hsiang [1 ]
Yang, Tinglu [1 ]
Wark, Stacey E. [1 ]
Son, Dong Hee [1 ]
Batteas, James D. [1 ]
机构
[1] Texas A&M Univ, Dept Chem, College Stn, TX 77842 USA
基金
美国国家科学基金会;
关键词
CDSE NANOCRYSTALS; PHOTOLUMINESCENCE; NANOPARTICLES; NANOASSEMBLIES; ENHANCEMENT; MONOLAYERS;
D O I
10.1021/ja906837s
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Photolithographically generated patterns have been created on immobilized CdSe QD thin films by fine-tuning their optical properties (intensity and emission wavelength) postsynthetically. These optically modified QDs show enhanced selectivity for binding of different ligands, affording the ability to fabricate optically reconfigurable surfaces for display or sensing applications. The patterns may be readily generated with any typical optical lithographic approach.
引用
收藏
页码:18204 / +
页数:3
相关论文
共 31 条
  • [1] Size-dependent dissociation pH of thiolate ligands from cadmium chalcogenide nanocrystals
    Aldana, J
    Lavelle, N
    Wang, YJ
    Peng, XG
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (08) : 2496 - 2504
  • [2] Photochemical instability of CdSe nanocrystals coated by hydrophilic thiols
    Aldana, J
    Wang, YA
    Peng, XG
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2001, 123 (36) : 8844 - 8850
  • [3] [Anonymous], J PHYS CHEM
  • [4] Kinetically driven self assembly of highly ordered nanoparticle monolayers
    Bigioni, TP
    Lin, XM
    Nguyen, TT
    Corwin, EI
    Witten, TA
    Jaeger, HM
    [J]. NATURE MATERIALS, 2006, 5 (04) : 265 - 270
  • [5] Optical biosensors
    Borisov, Sergey M.
    Wolfbeis, Otto S.
    [J]. CHEMICAL REVIEWS, 2008, 108 (02) : 423 - 461
  • [6] Semiconductor nanocrystals as fluorescent biological labels
    Bruchez, M
    Moronne, M
    Gin, P
    Weiss, S
    Alivisatos, AP
    [J]. SCIENCE, 1998, 281 (5385) : 2013 - 2016
  • [7] Quantum dots luminescence enhancement due to illumination with UV/Vis light
    Carrillo-Carrion, Carolina
    Cardenas, Soledad
    Simonet, Bartolome M.
    Valcarcel, Miguel
    [J]. CHEMICAL COMMUNICATIONS, 2009, (35) : 5214 - 5226
  • [8] Evaporation-Induced Assembly of Quantum Dots into Nanorings
    Chen, Jixin
    Liao, Wei-Ssu
    Chen, Xin
    Yang, Tinglu
    Wark, Stacey E.
    Son, Dong Hee
    Batteas, James D.
    Cremer, Paul S.
    [J]. ACS NANO, 2009, 3 (01) : 173 - 180
  • [9] Electroluminescence from single monolayers of nanocrystals in molecular organic devices
    Coe, S
    Woo, WK
    Bawendi, M
    Bulovic, V
    [J]. NATURE, 2002, 420 (6917) : 800 - 803
  • [10] Tunable nonlocal spin control in a coupled-quantum dot system
    Craig, NJ
    Taylor, JM
    Lester, EA
    Marcus, CM
    Hanson, MP
    Gossard, AC
    [J]. SCIENCE, 2004, 304 (5670) : 565 - 567