Destruction of humic acid in water by UV light - Catalyzed oxidation with hydrogen peroxide

被引:151
作者
Wang, GS
Hsieh, ST
Hong, CS
机构
[1] Natl Taiwan Univ, Dept Publ Hlth, Taipei, Taiwan
[2] New York State Dept Hlth, Wadsworth Ctr Labs & Res, Albany, NY 12201 USA
关键词
humic acid; hydrogen peroxide (H2O2); advanced oxidation process (AOP);
D O I
10.1016/S0043-1354(00)00120-2
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A batch reactor was used to evaluate the advanced oxidation process of the UV/H2O2 system for control of natural organic matter (NOM) in drinking water. The light sources used include a 450 W high-pressure mercury vapor lamp and sunlight. Both quartz and Pyrex filters were used to control the wavelength and energy of UV light applied to the aqueous systems. The results showed that NOM oxidation and H2O2 decomposition followed first-order and zero-order reaction kinetics, respectively. The optimum H2O2 dose was found to be 0.01% for the oxidation of humic acids in this study. Carbonate and bicarbonate ions inhibited the degradation of humic acids. (C) 2000 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:3882 / 3887
页数:6
相关论文
共 26 条
[11]   CRITICAL-REVIEW OF RATE CONSTANTS FOR REACTIONS OF HYDRATED ELECTRONS, HYDROGEN-ATOMS AND HYDROXYL RADICALS (.OH/.O-) IN AQUEOUS-SOLUTION [J].
BUXTON, GV ;
GREENSTOCK, CL ;
HELMAN, WP ;
ROSS, AB .
JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA, 1988, 17 (02) :513-886
[12]   Photocatalytic treatment of humic substances in drinking water [J].
Eggins, BR ;
Palmer, FL ;
Byrne, JA .
WATER RESEARCH, 1997, 31 (05) :1223-1226
[13]   ADVANCED OXIDATION PROCESSES - A KINETIC-MODEL FOR THE OXIDATION OF 1,2-DIBROMO-3-CHLOROPROPANE IN WATER BY THE COMBINATION OF HYDROGEN-PEROXIDE AND UV-RADIATION [J].
GLAZE, WH ;
LAY, Y ;
KANG, JW .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1995, 34 (07) :2314-2323
[14]   PREOZONATION OF CHLOROPHENOLIC WASTE-WATER FOR SUBSEQUENT BIOLOGICAL TREATMENT [J].
HU, ST ;
YU, YH .
OZONE-SCIENCE & ENGINEERING, 1994, 16 (01) :13-28
[15]   THE PHOTOCHEMICAL DECOMPOSITION OF HYDROGEN PEROXIDE - QUANTUM YIELDS, TRACER AND FRACTIONATION EFFECTS [J].
HUNT, JP ;
TAUBE, H .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1952, 74 (23) :5999-6002
[16]  
JACANGELO JG, 1995, J AM WATER WORKS ASS, V87, P64
[17]   A kinetic model of the hydrogen peroxide UV process for the treatment of hazardous waste chemicals [J].
Kang, JW ;
Le, KH .
ENVIRONMENTAL ENGINEERING SCIENCE, 1997, 14 (03) :183-192
[18]  
Ku Y, 1998, J HAZARD MATER, V60, P41
[19]   CHEMICAL OXIDATION BY PHOTOLYTIC DECOMPOSITION OF HYDROGEN-PEROXIDE [J].
LIAO, CH ;
GUROL, MD .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1995, 29 (12) :3007-3014
[20]  
OWEN DM, 1995, J AM WATER WORKS ASS, V87, P46