Direct observation of the dynamics of excited electronic states in solids:: f-sec time resolved photoemission of C60

被引:35
作者
Jacquemin, R [1 ]
Kraus, S [1 ]
Eberhardt, W [1 ]
机构
[1] Forschungszentrum Julich, Inst Festkorperforsch, D-52425 Julich, Germany
关键词
fullerenes; electronic states; recombination and trapping; photoelectron spectroscopies; time-resolved optical spectroscopies;
D O I
10.1016/S0038-1098(97)10174-0
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Using femtosecond laser pulses in a pump-probe configuration we have studied the dynamics of optically excited states in C-60 films deposited onto a metallic substrate. The excited electrons are observed directly by taking photoemission spectra while varying the time-delay between pump and probe pulses. The initially excited electronic configurations which are reached from the ground state via dipole transitions decay with different time constants into lower energy configurations. (C) 1998 Elsevier Science Ltd.
引用
收藏
页码:449 / 453
页数:5
相关论文
共 20 条
  • [1] PULSED EPR ON THE PHOTOEXCITED TRIPLET-STATE OF C(60)-FULLERENE
    BENNATI, M
    GRUPP, A
    MEHRING, M
    DINSE, KP
    FINK, J
    [J]. CHEMICAL PHYSICS LETTERS, 1992, 200 (05) : 440 - 444
  • [2] TIME-RESOLVED AND ANGLE-RESOLVED PHOTOEMISSION-STUDY OF INP(110)
    BOKOR, J
    HAIGHT, R
    STORZ, RH
    STARK, J
    FREEMAN, RR
    BUCKSBAUM, PH
    [J]. PHYSICAL REVIEW B, 1985, 32 (06): : 3669 - 3675
  • [3] BOKOR J, 1985, PHYS REV LETT, V54, P1302
  • [4] FEMTOSECOND PUMP-PROBE INVESTIGATION OF ELECTRON DYNAMICS IN SOLID C-60 FILMS
    BRORSON, SD
    KELLY, MK
    WENSCHUH, U
    BUHLEIER, R
    KUHL, J
    [J]. PHYSICAL REVIEW B, 1992, 46 (11): : 7329 - 7332
  • [5] TIME-RESOLVED PHOTOLUMINESCENCE OF SOLID-STATE FULLERENES
    BYRNE, HJ
    MASER, W
    RUHLE, WW
    MITTELBACH, A
    HONLE, W
    VONSCHNERING, HG
    MOVAGHAR, B
    ROTH, S
    [J]. CHEMICAL PHYSICS LETTERS, 1993, 204 (5-6) : 461 - 466
  • [6] HIGH-RESOLUTION ELECTRON-ENERGY-LOSS SPECTROSCOPY OF THIN-FILMS OF C60 ON SI(100)
    GENSTERBLUM, G
    PIREAUX, JJ
    THIRY, PA
    CAUDANO, R
    VIGNERON, JP
    LAMBIN, P
    LUCAS, AA
    KRATSCHMER, W
    [J]. PHYSICAL REVIEW LETTERS, 1991, 67 (16) : 2171 - 2174
  • [7] PREPARATION AND UV VISIBLE SPECTRA OF FULLERENES C60 AND C70
    HARE, JP
    KROTO, HW
    TAYLOR, R
    [J]. CHEMICAL PHYSICS LETTERS, 1991, 177 (4-5) : 394 - 398
  • [8] ITCHKAWITZ BS, 1995, P 22 INT C PHYS SEM, V3, P2057
  • [9] INTERMOLECULAR CHARGE-TRANSFER EXCITATION IN C-60 FILMS - EVIDENCE FROM LUMINESCENCE AND PHOTOCONDUCTIVITY
    KAZAOUI, S
    ROSS, R
    MINAMI, N
    [J]. PHYSICAL REVIEW B, 1995, 52 (16) : 11665 - 11668
  • [10] KAZAOUI S, 1995, P INT WINT EL PROP N