Pressure drop measurements and modeling on SiC foams

被引:241
作者
Lacroix, Maxime
Nguyen, Patrick
Schweich, Daniel
Huu, Cuong Pham
Savin-Poncet, Sabine
Edouard, David
机构
[1] Univ Strasbourg, ELCASS, LMSPC, CNRS,ECPM,UMR 7515, F-67087 Strasbourg, France
[2] SiCat Tech Ctr, F-67700 Otterswiller, France
[3] LGPC, CPE 43, F-69616 Villeurbanne, France
[4] Ctr Sci & Tech Jean Feger, TOTAL, F-64000 Pau, France
关键词
pressure drop; foam; cubic lattice model; catalysis; silicon carbide; Ergun equation;
D O I
10.1016/j.ces.2007.03.027
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Foam-structured beds are likely to be the next generation of catalyst supports due to their interesting specific properties (large exchange area, low pressure drop, easy control of external porosity, etc.). Nevertheless, chemical engineering parameters of this new catalyst support types are still not completely clear for the scientific community and many approaches are attempted to solve this problem. SiC foams offer the dual advantages of the interesting properties of structured beds and the intrinsic thermal and mechanical properties of silicon carbide as a catalytic support. In the present work, the problem of pressure drops along foam beds is studied with a new simplistic geometrical model as a first step in the understanding of the peculiar hydrodynamic behavior of SiC foams in chemical processes. The proposed model was successfully validated by experimental results on a relatively large range of parameters which fully confirm the validity of the model. (c) 2007 Elsevier Ltd. All rights reserved.
引用
收藏
页码:3259 / 3267
页数:9
相关论文
共 29 条
[1]   Pd-Ag/SiO2 xerogel catalyst forming by impregnation on alumina foams [J].
Alié, C ;
Ferauche, F ;
Léonard, A ;
Lambert, S ;
Tcherkassova, N ;
Heinrichs, B ;
Crine, M ;
Marchot, P ;
Loukine, E ;
Pirard, JP .
CHEMICAL ENGINEERING JOURNAL, 2006, 117 (01) :13-22
[2]   NON-DARCY FLOW THEOUGH FIBROUS POROUS MEDIA [J].
BEAVERS, GS ;
SPARROW, EM .
JOURNAL OF APPLIED MECHANICS, 1969, 36 (04) :711-&
[3]   Thermophysical properties of high porosity metal foams [J].
Bhattacharya, A ;
Calmidi, VV ;
Mahajan, RL .
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2002, 45 (05) :1017-1031
[4]   Ceramic foam monoliths as catalyst carriers. 1. Adjustment and description of the morphology [J].
Buciuman, FC ;
Kraushaar-Czarnetzki, B .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2003, 42 (09) :1863-1869
[5]   AN ASSESSMENT OF EXPRESSIONS FOR THE APPARENT THERMAL-CONDUCTIVITY OF CELLULAR MATERIALS [J].
COLLISHAW, PG ;
EVANS, JRG .
JOURNAL OF MATERIALS SCIENCE, 1994, 29 (02) :486-498
[6]  
ERGUN S, 1952, CHEM ENG PROGR, V48, P2
[7]  
Fourie JG, 2002, CHEM ENG SCI, V57, P2781
[8]   Mass-transfer characterization of metallic foams as supports for structured catalysts [J].
Giani, L ;
Groppi, G ;
Tronconi, E .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2005, 44 (14) :4993-5002
[9]  
GIBSON LJ, 1997, CELLULAR SOLIDS
[10]   Design of novel monolith catalyst supports for gas/solid reactions with heat exchange [J].
Groppi, G ;
Tronconi, E .
CHEMICAL ENGINEERING SCIENCE, 2000, 55 (12) :2161-2171