Scattering indued optical limiting in Si/SiO2 nanostructure dispersions

被引:23
作者
King, Sharon M. [1 ]
Chaure, Shweta
Doyle, James
Colli, Alan
Ferrari, Andrea C.
Blau, Werner J.
机构
[1] Univ Dublin Trinity Coll, Sch Phys, Dublin 2, Ireland
[2] Univ Cambridge, Ctr Adv Photon & Elect, Cambridge CB2 1TN, England
关键词
D O I
10.1016/j.optcom.2007.04.028
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We present evidence for scattering induced optical limiting in a suspension of Si/SiO2 nanostructures in an isopropanol solution. The structures were studied by open and closed aperture z-scan with 6 ns Gaussian pulses at 532 nm from a frequency doubled, Q switched Nd:YAG laser. The linear absorption of the nanostructures displayed evidence of quantum confinement. An intensity dependent scattering study illustrated the contribution to optical limiting from scattering mechanisms. We propose that optical limiting is occurring at scattering centres, most likely plasmas, which are formed through ionisation of the SiO2 outer shells. (c) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码:305 / 309
页数:5
相关论文
共 27 条
  • [1] MECHANISM FOR ENHANCED OPTICAL NONLINEARITIES AND BISTABILITY BY COMBINED DIELECTRIC ELECTRONIC CONFINEMENT IN SEMICONDUCTOR MICROCRYSTALLITES
    CHEMLA, DS
    MILLER, DAB
    [J]. OPTICS LETTERS, 1986, 11 (08) : 522 - 524
  • [2] Modified carbon nanotubes as broadband optical limiting nanomaterials
    Chin, Kok Chung
    Gohel, Amarsinh
    Elim, Hendry Izaac
    Chen, Weizhe
    Ji, Wei
    Chong, Ghee Lee
    Sow, Chorng Haur
    Wee, Andrew T. S.
    [J]. JOURNAL OF MATERIALS RESEARCH, 2006, 21 (11) : 2758 - 2766
  • [3] Synthesis and optical properties of silicon nanowires grown by different methods
    Colli, A.
    Hofmann, S.
    Fasoli, A.
    Ferrari, A. C.
    Ducati, C.
    Dunin-Borkowski, R. E.
    Robertson, J.
    [J]. APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 2006, 85 (03): : 247 - 253
  • [4] LASER-INDUCED BREAKDOWN BY IMPACT IONIZATION IN SIO2 WITH PULSE WIDTHS FROM 7 NS TO 150 FS
    DU, D
    LIU, X
    KORN, G
    SQUIER, J
    MOUROU, G
    [J]. APPLIED PHYSICS LETTERS, 1994, 64 (23) : 3071 - 3073
  • [5] Picosecond-resolution study of nonlinear scattering in carbon black suspensions in water and ethanol
    Durand, O
    Grolier-Mazza, V
    Frey, R
    [J]. OPTICS LETTERS, 1998, 23 (18) : 1471 - 1473
  • [6] FEIN A, 1994, 3 FRENCH ISR S NON L
  • [7] FOX M, 2001, OPTICAL PROPERTIES S, P66
  • [8] Excitonic nonlinear absorption in CdS nanocrystals studied using Z-scan technique
    He, J
    Ji, W
    Ma, GH
    Tang, SH
    Elim, HI
    Sun, WX
    Zhang, ZH
    Chin, WS
    [J]. JOURNAL OF APPLIED PHYSICS, 2004, 95 (11) : 6381 - 6386
  • [9] Highly luminescent silicon nanocrystals with discrete optical transitions
    Holmes, JD
    Ziegler, KJ
    Doty, RC
    Pell, LE
    Johnston, KP
    Korgel, BA
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2001, 123 (16) : 3743 - 3748
  • [10] Characterization of nonlinear scattering in colloidal suspensions of silica particles
    Joudrier, V
    Bourdon, P
    Hache, F
    Flytzanis, C
    [J]. APPLIED PHYSICS B-LASERS AND OPTICS, 2000, 70 (01): : 105 - 109