Moisture assisted perovskite film growth for high performance solar cells

被引:667
作者
You, Jingbi [1 ]
Yang, Yang [1 ]
Hong, Ziruo [1 ]
Song, Tze-Bin [1 ]
Meng, Lei [1 ]
Liu, Yongsheng [1 ]
Jiang, Chengyang [1 ]
Zhou, Huanping [1 ]
Chang, Wei-Hsuan [1 ]
Li, Gang [1 ]
Yang, Yang [1 ,2 ]
机构
[1] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA
[2] Univ Calif Los Angeles, Calif NanoSyst Inst, Los Angeles, CA 90095 USA
基金
美国国家科学基金会;
关键词
HIGH-EFFICIENCY; LOW-COST; WATER; LENGTHS;
D O I
10.1063/1.4901510
中图分类号
O59 [应用物理学];
学科分类号
摘要
Moisture is assumed to be detrimental to organometal trihalide perovskite, as excess water can damage the crystallinity of the perovskite structure. Here, we report a growth mode for via thermal annealing of the perovskite precursor film in a humid environment (e. g., ambient air) to greatly improve the film quality, grain size, carrier mobility, and lifetime. Our method produces devices with maximum power conversion efficiency of 17.1% and a fill factor of 80%, revealing a promising route to achieve high quality perovskite polycrystalline films with superior optoelectronic properties that can pave the way towards efficient photovoltaic conversion. (C) 2014 AIP Publishing LLC.
引用
收藏
页数:5
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