Ammonia-Treated Ordered Mesoporous Carbons as Catalytic Materials for Oxygen Reduction Reaction

被引:331
作者
Wang, Xiqing [1 ]
Lee, Je Seung [1 ]
Zhu, Qing [1 ]
Liu, Jun [2 ]
Wang, Yong [2 ]
Dai, Sheng [1 ]
机构
[1] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA
[2] Pacific NW Natl Lab, Richland, WA 99352 USA
关键词
ELECTROLYTE FUEL-CELLS; NITROGEN-CONTAINING CARBON; ACTIVE-SITES; SUPPORT; METAL; ELECTROCATALYST; SPECTROSCOPY; ENHANCEMENT; TEMPERATURE; DURABILITY;
D O I
10.1021/cm100139d
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Ammonia treatment of ordered mesoporous carbons at high temperature results in the formation of nitrogen-doped carbon materials that exhibit significant activity for oxygen reduction reaction in acidic media. The new material shows an onset potential of only 80 mV below that of a commercial Pt-based catalyst, but a better stability. © 2010 American Chemical Society.
引用
收藏
页码:2178 / 2180
页数:3
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