Free carrier generation in semiconductors induced by absorption of subband-gap light

被引:20
作者
Vanmaekelbergh, D [1 ]
van Pieterson, L [1 ]
机构
[1] Univ Utrecht, Debye Inst, NL-3508 TA Utrecht, Netherlands
关键词
D O I
10.1103/PhysRevLett.80.821
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The mechanisms of electron-hole pair generation in a semiconductor induced by absorption of a subband-gap photon and mediated by a band-gap state are reviewed. The steady-state photocurrent quantum yield and the photocurrent response to harmonic modulation of the light intensity are calculated for each mechanism. It is shown, with a nanoporous GaP photoanode as an example, that the mechanisms can be distinguished by intensity-modulated photocurrent spectroscopy and that characterization of the mediating band-gap states is possible.
引用
收藏
页码:821 / 824
页数:4
相关论文
共 13 条
[1]   PHOTOEXCITATION AND LUMINESCENCE IN REDOX PROCESSES ON GALLIUM PHOSPHIDE ELECTRODES [J].
BECKMANN, KH ;
MEMMING, R .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1969, 116 (03) :368-&
[2]   SURFACE-STATES INDUCED BY METAL ATOMS AT THE SI ELECTROLYTE INTERFACE [J].
CHAZALVIEL, JN ;
STEFENEL, M ;
TRUONG, TB .
SURFACE SCIENCE, 1983, 134 (03) :865-885
[3]   OPTICAL DETECTION OF SURFACE STATES ON CLEAVED (111) SURFACES OF GE [J].
CHIAROTTI, G ;
DELSIGNO.G ;
NANNARONE, S .
PHYSICAL REVIEW LETTERS, 1968, 21 (16) :1170-+
[4]   Trap-limited electronic transport in assemblies of nanometer-size TiO2 particles [J].
de Jongh, PE ;
Vanmaekelbergh, D .
PHYSICAL REVIEW LETTERS, 1996, 77 (16) :3427-3430
[5]   POROUS ETCHING - A MEANS TO ENHANCE THE PHOTORESPONSE OF INDIRECT SEMICONDUCTORS [J].
ERNE, BH ;
VANMAEKELBERGH, D ;
KELLY, JJ .
ADVANCED MATERIALS, 1995, 7 (08) :739-742
[6]   PERSISTENT PHOTOCONDUCTANCE IN N-TYPE 6H-SIC [J].
EVWARAYE, AO ;
SMITH, SR ;
MITCHEL, WC .
JOURNAL OF APPLIED PHYSICS, 1995, 77 (09) :4477-4481
[7]   SEMICONDUCTOR SURFACE SPECTROSCOPIES - THE EARLY YEARS [J].
LAGOWSKI, J .
SURFACE SCIENCE, 1994, 299 (1-3) :92-101
[8]   Greatly enhanced sub-bandgap photocurrent in porous GaP photoanodes [J].
Marin, FI ;
Hamstra, MA ;
Vanmaekelbergh, D .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1996, 143 (03) :1137-1142
[9]   Modulation spectroscopy of subbandgap light in reduced TiO2 electrodes [J].
Nogami, G ;
Ohkubo, S ;
Avalle, L ;
Hongo, K .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1996, 143 (11) :3600-3606
[10]  
Pankove J., 1975, OPTICAL PROCESSES SE