Characterization and temporal variation of Asian dust aerosol from a site in the northern Chinese deserts

被引:114
作者
Zhang, XY
Gong, SL
Arimoto, R
Shen, ZX
Mei, FM
Wang, D
Cheng, Y
机构
[1] Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian 710075, Peoples R China
[2] Meteorol Serv Canada, ARQM, Toronto, ON M3H 5T4, Canada
[3] New Mexico State Univ, Carlsbad Environm Monitoring & Res Ctr, Carlsbad, NM 88220 USA
基金
中国国家自然科学基金; 美国国家科学基金会;
关键词
Asian dust; Chinese deserts; dust storm; elements; size distribution;
D O I
10.1023/A:1022900220357
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Time series for total aerosol mass and the concentrations of nineteen elements, and the mass particle-size distributions of the elements, were determined for samples collected from a site in the northern deserts of China-Zhenbeitai, one of ground sites of the Asia-Pacific Regional Aerosol Characterization Experiment ( ACE-Asia). Nine dust storm (DS) events were observed during the spring of 2001, lasting a combined total of twenty-six days. Peak mass loadings greatly exceeded the average (260 mug m(-3)), and higher than average dust-element concentrations and wind speeds were also observed during the three-month study. Material balance calculations showed that similar to82% mass of the total aerosol particles could be ascribed to Asian dust, of which Al, Ca, Fe, K, Mn, Si and Ti accounted for 7%, 6%, 4%, 2%, 0.1%, 32% and 1% by weight, respectively. Modelcalculated dry deposition velocities for 7 dust-elements during dust storm periods averaged 17 cm s(-1) and ranged from 14 to 21 cm s(-1). The estimated dry depositiona of Asian dust for the spring of 2001 was 189 g m(-2), of which 85% was due to dust storms. Factor analysis indicated that similar to89% of the dust loading during this period was due to remote or regional transport; similar to11% to local or background dust.
引用
收藏
页码:241 / 257
页数:17
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