Double-Resonance Plasmon Substrates for Surface-Enhanced Raman Scattering with Enhancement at Excitation and Stokes Frequencies

被引:256
作者
Chu, Yizhuo [1 ]
Banaee, Mohamad G. [1 ]
Crozier, Kenneth B. [1 ]
机构
[1] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA
基金
美国国家科学基金会;
关键词
localized surface plasmon; surface plasmon polariton; nanoparticle; surface enhanced Raman scattering; spatial distribution; hybridization;
D O I
10.1021/nn901826q
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report a surface-enhanced Raman scattering (SERS) substrate with plasmon resonances at both excitation and Stokes frequencies. This multilayer structure combines localized surface plasmons on the nanoparticles with surface plasmon polaritons excited on a gold film. The largest SERS enhancement factor for a gold device is measured to be 7.2 x 10(7), which is more than 2 orders of magnitude larger than that measured on a gold nanoparticle array on a glass substrate. The largest SERS enhancement for a silver device is measured to be 8.4 x 10(8).
引用
收藏
页码:2804 / 2810
页数:7
相关论文
共 26 条
[1]   Optical properties of gold nanorings -: art. no. 057401 [J].
Aizpurua, J ;
Hanarp, P ;
Sutherland, DS ;
Käll, M ;
Bryant, GW ;
de Abajo, FJG .
PHYSICAL REVIEW LETTERS, 2003, 90 (05) :4
[2]   Gold nanorings as substrates for surface-enhanced Raman scattering [J].
Banaee, Mohamad G. ;
Crozier, Kenneth B. .
OPTICS LETTERS, 2010, 35 (05) :760-762
[3]   Investigation of surface-enhanced Raman scattering from platinum electrodes using a confocal Raman microscope: dependence of surface roughening pretreatment [J].
Cai, WB ;
Ren, B ;
Li, XQ ;
She, CX ;
Liu, FM ;
Cai, XW ;
Tian, ZQ .
SURFACE SCIENCE, 1998, 406 (1-3) :9-22
[4]   Experimental observation of narrow surface plasmon resonances in gold nanoparticle arrays [J].
Chu, Yizhuo ;
Schonbrun, Ethan ;
Yang, Tian ;
Crozier, Kenneth B. .
APPLIED PHYSICS LETTERS, 2008, 93 (18)
[5]   Experimental study of the interaction between localized and propagating surface plasmons [J].
Chu, Yizhuo ;
Crozier, Kenneth B. .
OPTICS LETTERS, 2009, 34 (03) :244-246
[6]   Gold particle interaction in regular arrays probed by surface enhanced Raman scattering [J].
Félidj, N ;
Truong, SL ;
Aubard, J ;
Lévi, G ;
Krenn, JR ;
Hohenau, A ;
Leitner, A ;
Aussenegg, FR .
JOURNAL OF CHEMICAL PHYSICS, 2004, 120 (15) :7141-7146
[7]   Optical properties of periodic structures of metallic nanodisks [J].
Gantzounis, G. ;
Stefanou, N. ;
Papanikolaou, N. .
PHYSICAL REVIEW B, 2008, 77 (03)
[8]   Experimental observation of mode-selective anticrossing in surface-plasmon-coupled metal nanoparticle arrays [J].
Ghoshal, Amitabh ;
Divliansky, Ivan ;
Kik, Pieter G. .
APPLIED PHYSICS LETTERS, 2009, 94 (17)
[9]   Role of localized surface plasmons in surface-enhanced Raman scattering of shape-controlled metallic particles in regular arrays [J].
Grand, J ;
de la Chapelle, ML ;
Bijeon, JL ;
Adam, PM ;
Vial, A ;
Royer, P .
PHYSICAL REVIEW B, 2005, 72 (03)
[10]   Plasmon-sampled surface-enhanced Raman excitation spectroscopy [J].
Haynes, CL ;
Van Duyne, RP .
JOURNAL OF PHYSICAL CHEMISTRY B, 2003, 107 (30) :7426-7433