Optical analysis of nanoparticles via enhanced backscattering facilitated by 3-D photonic nanojets

被引:307
作者
Li, X [1 ]
Chen, ZG
Taflove, A
Backman, V
机构
[1] Northwestern Univ, Dept Biomed Engn, Evanston, IL 60208 USA
[2] Northwestern Univ, Dept Elect & Comp Engn, Evanston, IL 60208 USA
来源
OPTICS EXPRESS | 2005年 / 13卷 / 02期
关键词
D O I
10.1364/OPEX.13.000526
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We report the phenomenon of ultra-enhanced backscattering of visible light by nanoparticles facilitated by the 3-D photonic nanojet - a sub-diffraction light beam appearing at the shadow side of a plane-wave-illuminated dielectric microsphere. Our rigorous numerical simulations show that backscattering intensity of nanoparticles can be enhanced up to eight orders of magnitude when locating in the nanojet. As a result, the enhanced backscattering from a nanoparticle with diameter on the order of 10 nm is well above the background signal generated by the dielectric microsphere itself. We also report that nanojet-enhanced backscattering is extremely sensitive to the size of the nanoparticle, permitting in principle resolving sub-nanometer size differences using visible light. Finally, we show how the position of a nanoparticle could be determined with subdiffractional accuracy by recording the angular distribution of the backscattered light. These properties of photonic nanojets promise to make this phenomenon a useful tool for optically detecting, differentiating, and sorting nanoparticles. (C) 2005 Optical Society of America.
引用
收藏
页码:526 / 533
页数:8
相关论文
共 12 条
[1]   Measuring cellular structure at submicrometer scale with light scattering spectroscopy [J].
Backman, V ;
Gopal, V ;
Kalashnikov, M ;
Badizadegan, K ;
Gurjar, R ;
Wax, A ;
Georgakoudi, I ;
Mueller, M ;
Boone, CW ;
Dasari, RR ;
Feld, MS .
IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS, 2001, 7 (06) :887-893
[2]   SPATIAL-DISTRIBUTION OF THE INTERNAL AND NEAR-FIELD INTENSITIES OF LARGE CYLINDRICAL AND SPHERICAL SCATTERERS [J].
BENINCASA, DS ;
BARBER, PW ;
ZHANG, JZ ;
HSIEH, WF ;
CHANG, RK .
APPLIED OPTICS, 1987, 26 (07) :1348-1356
[3]  
Bohren C., 1983, ABSORPTION SCATTERIN
[4]   Photonic nanojet enhancement of backscattering of light by nanoparticles: a potential novel visible-light ultramicroscopy technique [J].
Chen, ZG ;
Taflove, A ;
Backman, V .
OPTICS EXPRESS, 2004, 12 (07) :1214-1220
[5]   INTERNAL AND NEAR-SURFACE SCATTERED FIELD OF A SPHERICAL-PARTICLE AT RESONANT CONDITIONS [J].
CHYLEK, P ;
PENDLETON, JD ;
PINNICK, RG .
APPLIED OPTICS, 1985, 24 (23) :3940-3942
[6]   Focusing in microlenses close to a wavelength in diameter [J].
Fletcher, DA ;
Goodson, KE ;
Kino, GS .
OPTICS LETTERS, 2001, 26 (07) :399-401
[7]   Cooperative microlenses [J].
Helseth, LE ;
Fischer, TM .
OPTICS EXPRESS, 2004, 12 (15) :3428-3435
[8]   OPTICAL CONSTANTS OF NOBLE METALS [J].
JOHNSON, PB ;
CHRISTY, RW .
PHYSICAL REVIEW B, 1972, 6 (12) :4370-4379
[9]   SCATTERING BY 2 SPHERES [J].
LIANG, C ;
LO, YT .
RADIO SCIENCE, 1967, 2 (12) :1481-+
[10]   Optical field enhancement effects in laser-assisted particle removal [J].
Mosbacher, M ;
Münzer, HJ ;
Zimmermann, J ;
Solis, J ;
Boneberg, J ;
Leiderer, P .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 2001, 72 (01) :41-44