Large off-diagonal magnetoelectric coupling in the quantum paraelectric antiferromagnet EuTiO3

被引:91
作者
Shvartsman, V. V. [1 ]
Borisov, P. [1 ]
Kleemann, W. [1 ]
Kamba, S. [2 ]
Katsufuji, T. [3 ]
机构
[1] Univ Duisburg Essen, D-47048 Duisburg, Germany
[2] ASCR, Inst Phys, Prague 18221 8, Czech Republic
[3] Waseda Univ, Dept Phys, Shinjuku Ku, Tokyo 1698555, Japan
关键词
SUSCEPTIBILITY; BIREFRINGENCE; SYMMETRY;
D O I
10.1103/PhysRevB.81.064426
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The third-order (EH2)-H-2-type magnetoelectric (ME) response of polycrystalline EuTiO3 changes sign under magnetic bias and shows a large anomaly at the antiferromagnetic (AF)-paramagnetic phase boundary below T-N approximate to 5.3 K. It is attributed to critical fluctuations of the AF order parameter reinforced by quantum paraelectric polar correlations. The underlying biquadratic spin-lattice coupling involves electric field induced Dzyaloshinskii-Moriya interaction as described within mean-field approximation. Single domaining by ME annealing (or cooling) significantly enhances the response by additional EH and EH2 effects.
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页数:4
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