Size effects in the electronic properties of finite arrays of exchange-coupled quantum dots

被引:12
作者
Wang, JX
Kais, S
Remacle, F
Levine, RD [1 ]
机构
[1] Hebrew Univ Jerusalem, Fritz Haber Res Ctr Mol Dynam, IL-91904 Jerusalem, Israel
[2] Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA
[3] Univ Liege, Dept Chem, B-4000 Liege, Belgium
关键词
D O I
10.1021/jp026452a
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Transport properties of arrays of metallic quantum dots are governed by the distance-dependent exchange coupling between the dots. It is shown that the effective value of the exchange coupling, as measured by the charging energy per dot, depends monotonically on the size of the array. The effect saturates for-hexagonal arrays of over 7(5) unit cells. The discussion uses a multistage block renormalization group approach applied to the Hubbard Hamiltonian. A first-order phase transition occurs upon compression of the lattice, and the size dependence is qualitatively different for the two phases.
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页码:12847 / 12850
页数:4
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