Preparation and characterization of Ag/MnOx/perovskite catalysts for CO oxidation

被引:63
作者
Song, KS
Kang, SK
Kim, SD
机构
[1] Korea Inst Energy Res, Catalyt Combust Res Team, Taejon 305343, South Korea
[2] Korea Adv Inst Sci & Technol, Dept Chem Engn, Taejon 305701, South Korea
关键词
Ag; perovskite; CO oxidation; spray decomposition; Ag/MnOx/LaMnO3;
D O I
10.1023/A:1019072314394
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The spray decomposition method with lanthanum nitrate, manganese nitrate, silver nitrate and citric acid was used to synthesize Ag-and Mn-incorporated perovskites. The resulting samples were characterized by X-ray diffraction, BET adsorption measurement, X-ray photoelectron spectroscopy, and temperature-programmed oxygen desorption (O-2-TPD) measurement. The obtained composite Ag/MnOx/perovskites catalysts exhibit higher activity by a few orders of magnitude at 338 K than that of LaMnO3. From the O-2-TPD measurement, the high activity of the Ag/MnOx/perovskites may result from the increase of weak oxygen adsorption below 373 K.
引用
收藏
页码:65 / 68
页数:4
相关论文
共 18 条
[11]  
SONG KS, 1996, P 3 INT WORKSH CAT C
[12]  
Tabata K., 1990, CATAL TODAY, V8, P249, DOI [10.1016/0920-5861(90)87021-T, DOI 10.1016/0920-5861(90)87021-T]
[13]   PREPARATION, CHARACTERIZATION AND CATALYTIC PROPERTIES OF LAMEO3 OXIDES [J].
TASCON, JMD ;
MENDIOROZ, S ;
TEJUCA, LG .
ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-WIESBADEN, 1981, 124 (01) :109-127
[14]   STRUCTURE AND REACTIVITY OF PEROVSKITE-TYPE OXIDES [J].
TEJUCA, LG ;
FIERRO, JLG ;
TASCON, JMD .
ADVANCES IN CATALYSIS, 1989, 36 :237-328
[15]  
VISWANATHAN B, 1993, PROPERTIES APPL PERO, pCH13
[16]   DEFECT CHEMISTRY AND CATALYSIS IN OXIDATION AND REDUCTION OVER PEROVSKITE-TYPE OXIDES [J].
VOORHOEVE, RJH ;
REMEIKA, JP ;
TRIMBLE, LE .
ANNALS OF THE NEW YORK ACADEMY OF SCIENCES, 1976, 272 (APR28) :3-21
[17]  
Yamazoe N., 1990, Catalysis Today, V8, P175, DOI DOI 10.1016/0920-5861(90)87017-W
[18]   OXYGEN SORPTION AND CATALYTIC PROPERTIES OF LA1-XSRXCO1-YFEYO3 PEROVSKITE-TYPE OXIDES [J].
ZHANG, HM ;
SHIMIZU, Y ;
TERAOKA, Y ;
MIURA, N ;
YAMAZOE, N .
JOURNAL OF CATALYSIS, 1990, 121 (02) :432-440