NONLINEAR OPTICAL-PROPERTIES OF H-2 AND D-2

被引：33

作者：

BISHOP, DM

PIPIN, J

RERAT, M

机构：

[1] Department of Chemistry, University of Ottawa, Ottawa

[2] Equipe de Recherche (474) Associée au CNRS, Université de Pau

来源：

JOURNAL OF CHEMICAL PHYSICS | 1990年 / 92卷 / 03期

关键词：

D O I：

10.1063/1.458072

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Accurate wave functions of the James-Coolidge type, which account for electron correlation, are used to calculate for H2 and D2 the dynamic second hyperpolarizabilities (γ) which mediate the nonlinear optical processes: dc Kerr, dc electric-field-induced second-harmonic generation and third-harmonic generation. Values are given for a range of frequencies (ω = 0 to ω = 0.05 a.u.) as well as for some common laser frequencies. The effects of vibration are explicitly considered. As well, values of the dynamic field-gradient polarizabilities B and C are found. The results are more accurate than those previously published. © 1990 American Institute of Physics.

引用

页码：1902 / 1908

页数：7

共 25 条

[11] Bogaard M. P., 1975, INT REV SCI PHYS C 2, V2, P149
[12] Buckingham A. D., 1967, ADV CHEM PHYS, P107, DOI DOI 10.1002/9780470143582.CH2
[13] BIREFRINGENCE INDUCED IN SPHERICAL MOLECULES BY AN ELECTRIC FIELD GRADIENT
BUCKINGHAM, AD
JAMIESON, MJ
[J]. MOLECULAR PHYSICS, 1971, 22 (01) : 117 - +
[14] ELECTRIC BIREFRINGENCE IN MOLECULAR HYDROGEN
BUCKINGHAM, AD
ORR, BJ
[J]. PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1968, 305 (1481) : 259 - +
[15] MEASUREMENT OF THE KERR CONSTANT OF HE, A, O-2, N-2, H-2 AND D-2
CARUSOTTO, S
IACOPINI, E
POLACCO, E
SCURI, F
STEFANINI, G
ZAVATTINI, E
[J]. NUOVO CIMENTO DELLA SOCIETA ITALIANA DI FISICA D-CONDENSED MATTER ATOMIC MOLECULAR AND CHEMICAL PHYSICS FLUIDS PLASMAS BIOPHYSICS, 1985, 5 (04): : 328 - 338
[16] FINITE-FIELD MANY-BODY PERTURBATION-THEORY .4. BASIS SET OPTIMIZATION IN MBPT CALCULATIONS OF MOLECULAR-PROPERTIES - MOLECULAR QUADRUPOLE-MOMENTS
DIERCKSEN, GHF
SADLEJ, AJ
[J]. THEORETICA CHIMICA ACTA, 1983, 63 (01): : 69 - 82
[17] AN ABINITIO STUDY OF THE NON-LINEAR OPTICAL-PROPERTIES OF THE HE ATOM AND THE H-2 MOLECULE
JASZUNSKI, M
ROOS, BO
[J]. MOLECULAR PHYSICS, 1984, 52 (05) : 1209 - 1224
[18] HF SCF ELECTRIC POLARIZABILITIES AND HYPERPOLARIZABILITIES FOR THE GROUND-STATE OF THE HYDROGEN MOLECULE
MAROULIS, G
BISHOP, DM
[J]. CHEMICAL PHYSICS LETTERS, 1986, 128 (5-6) : 462 - 465
[19] FREQUENCY-DEPENDENT MULTIPOLE POLARIZABILITIES AND REDUCED GREENS FUNCTIONS .1. GROUND-STATE HYDROGEN-ATOM
MCDOWELL, K
[J]. JOURNAL OF CHEMICAL PHYSICS, 1977, 67 (05) : 1799 - 1806
[20] NONLINEAR SUSCEPTIBILITY OF H-2 AND D2 ACCURATELY MEASURED OVER A WIDE-RANGE OF WAVELENGTHS
MIZRAHI, V
SHELTON, DP
[J]. PHYSICAL REVIEW A, 1985, 32 (06): : 3454 - 3460

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