PHASE-EQUILIBRIUM FOR METHANE HYDRATE FROM 190-K TO 262-K

被引:84
作者
MAKOGON, TY [1 ]
SLOAN, ED [1 ]
机构
[1] COLORADO SCH MINES,CTR RES HYDRATES,GOLDEN,CO 80401
关键词
D O I
10.1021/je00014a035
中图分类号
O414.1 [热力学];
学科分类号
摘要
This work presents measurements on methane hydrate phase equilibrium in the three-phase region (ice + hydrate + vapor). Our results complement partial data sets from other laboratories and provide new results in the region 193-260 K. These data indicated that methane hydrate of structure I does not undergo a phase transition to structure II as proposed in recent literature.
引用
收藏
页码:351 / 353
页数:3
相关论文
共 14 条
[1]   HYDRATES OF HYDROCARBON GASES CONTAINING CARBON-DIOXIDE [J].
ADISASMITO, S ;
SLOAN, ED .
JOURNAL OF CHEMICAL AND ENGINEERING DATA, 1992, 37 (03) :343-349
[2]  
DEATON WM, 1946, BUREAU MINES MONOGR, P8
[3]  
Falabella B.J., 1975, THESIS U MASSACHUSET
[4]  
FRIEND DG, 1989, THERMOPHYSICAL PROPE, P156
[5]   CLATHRATE HYDRATES OF CYCLOPROPANE [J].
HAFEMANN, DR ;
MILLER, SL .
JOURNAL OF PHYSICAL CHEMISTRY, 1969, 73 (05) :1392-&
[7]  
HAWKINS RE, 1966, J PHYS CHEM-US, V79, P1889
[8]   MULTIPLE-PHASE EQUILIBRIA IN HYDRATES FROM METHANE, ETHANE, PROPANE AND WATER MIXTURES [J].
HOLDER, GD ;
HAND, JH .
AICHE JOURNAL, 1982, 28 (03) :440-447
[9]   CALCULATION OF PHASE-DIAGRAMS OF GAS-HYDRATES [J].
LUNDGAARD, L ;
MOLLERUP, J .
FLUID PHASE EQUILIBRIA, 1992, 76 :141-149
[10]   DIELECTRIC AND NUCLEAR MAGNETIC RESONANCE PROPERTIES OF A CLATHRATE HYDRATE OF CYCLOPROPANE [J].
MAJID, YA ;
GARG, SK ;
DAVIDSON, DW .
CANADIAN JOURNAL OF CHEMISTRY, 1969, 47 (24) :4697-&