POLARIZATION AND MATERIAL DEPENDENCE OF DEGENERATE 4-WAVE MIXING TRANSIENTS IN MOLECULAR FLUIDS

被引:12
作者
MCEWAN, KJ [1 ]
HARRISON, KJ [1 ]
MADDEN, PA [1 ]
机构
[1] UNIV OXFORD,PHYS CHEM LAB,OXFORD OX1 3QZ,ENGLAND
关键词
D O I
10.1080/00268979000100781
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The contributions of various microscopic mechanisms to the nonlinear optical response of molecular fluids are analysed for the case of degenerate four-wave mixing on the nanosecond timescale. A quantitative description of the transient responses obtained with different polarisation combinations is obtained. It is shown that this description applies well to experimental data gathered on a range of fluids and that molecular parameters that specify the amplitude and time dependence of the transients may be reliably measured. © 1990 Taylor & Francis Ltd.
引用
收藏
页码:1025 / 1042
页数:18
相关论文
共 18 条
[1]  
Berne B.J., 1976, DYNAMIC LIGHT SCATTE
[2]   A COMPREHENSIVE LIGHT-SCATTERING STUDY OF A LIQUID COMPOSED OF SYMMETRIC TOP MOLECULES [J].
CHAPPELL, PJ ;
KIVELSON, D .
JOURNAL OF CHEMICAL PHYSICS, 1982, 76 (04) :1742-1753
[3]  
DEGENNES PG, 1974, PHYSICS LIQUID CRYST
[4]   DIFFRACTION EFFICIENCY AND DECAY TIMES OF FREE-CARRIER GRATINGS IN SILICON [J].
EICHLER, HJ ;
MASSMANN, F .
JOURNAL OF APPLIED PHYSICS, 1982, 53 (04) :3237-3242
[5]   A PICOSECOND HOLOGRAPHIC GRATING APPROACH TO MOLECULAR-DYNAMICS IN ORIENTED LIQUID-CRYSTAL FILMS [J].
EYRING, G ;
FAYER, MD .
JOURNAL OF CHEMICAL PHYSICS, 1984, 81 (10) :4314-4321
[6]  
Fabelinskii IL, 1968, MOL SCATTERING LIGHT
[7]  
Fisher R.A., 2012, OPTICAL PHASE CONJUG
[8]  
HELLWARTH RW, 1977, PROG QUANT ELECTRON, V5, P1
[10]   LIGHT-SCATTERING-STUDIES OF MOLECULAR LIQUIDS [J].
KIVELSON, D ;
MADDEN, PA .
ANNUAL REVIEW OF PHYSICAL CHEMISTRY, 1980, 31 :523-558