PRONOUNCED CATALYTIC ACTIVITY OF FE0.08CS2.5H1.26PVMO11O40 FOR DIRECT OXIDATION OF PROPANE INTO ACRYLIC-ACID

被引:90
作者
MIZUNO, N [1 ]
TATEISHI, M [1 ]
IWAMOTO, M [1 ]
机构
[1] HOKKAIDO UNIV, CATALYSIS RES CTR, SAPPORO, HOKKAIDO 060, JAPAN
关键词
PROPANE; OXIDATION; ACRYLIC ACID; HETEROPOLY COMPOUNDS; IRON;
D O I
10.1016/0926-860X(95)00103-4
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Fe3+ or Ni2+-substitution for H+ and V5+-substitution for Mo6+ in, Cs2.5H0.5PMo12O40 greatly enhanced the catalytic activity for direct oxidation of propane into acrylic acid. Of the catalysts tested Cs2.5Fe0.08H1.26PVMo11O40 gave the highest yield of acrylic acid, 13%.
引用
收藏
页码:L165 / L170
页数:6
相关论文
共 32 条
[1]   OXIDATION OF PROPANE TO ACRYLIC-ACID ON V2O5-P2O5-BASED CATALYSTS [J].
AI, M .
JOURNAL OF CATALYSIS, 1986, 101 (02) :389-395
[2]  
AI M, 1985, 8TH P INT C CAT BERL, V5, P475
[4]   UNCHARGED ATOMIC OXYGEN IN OXIDATIVE CONVERSION OF C1-C2 ALKANES [J].
ANSHITS, AG .
CATALYSIS TODAY, 1992, 13 (04) :495-501
[5]  
ARTZ D, 1993, CATAL TODAY, V18, P173
[6]   HOMOGENEOUS AND HETEROGENEOUS CONTRIBUTIONS TO THE OXIDATIVE DEHYDROGENATION OF PROPANE ON OXIDE CATALYSTS [J].
BURCH, R ;
CRABB, EM .
APPLIED CATALYSIS A-GENERAL, 1993, 100 (01) :111-130
[7]  
CAVANI F, 1994, CHEMTECH APR, P18
[8]   FUNCTIONALIZATION OF ALKANES BY HETEROGENEOUS VAPOR-PHASE OXIDATION .2. PROPANE AMMOXIDATION [J].
CENTI, G ;
PESHEVA, D ;
TRIFIRO, F .
APPLIED CATALYSIS, 1987, 33 (02) :343-359
[9]   ACTIVE FORM OF 12-VANADOMOLYBDOPHOSPHORIC ACIDS IN NORMAL-BUTANE SELECTIVE OXIDATION [J].
CENTI, G ;
LENA, V ;
TRIFIRO, F ;
GHOUSSOUB, D ;
AISSI, CF ;
GUELTON, M ;
BONNELLE, JP .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS, 1990, 86 (15) :2775-2782
[10]   SELECTIVE OXIDATION OF NORMAL-PENTANE ON 12-MOLYBDOVANADOPHOSPHORIC ACIDS [J].
CENTI, G ;
NIETO, JL ;
IAPALUCCI, C ;
BRUCKMAN, K ;
SERWICKA, EM .
APPLIED CATALYSIS, 1989, 46 (02) :197-212