NEAR-THRESHOLD SITE-SELECTED DISSOCIATIVE IONIZATION OF CORE-EXCITED CARBON-DIOXIDE

被引:15
作者
HATHERLY, PA
CODLING, K
STANKIEWICZ, M
ROPER, M
机构
[1] JAGIELLONIAN UNIV,INST PHYS,PL-30059 KRAKOW,POLAND
[2] DARESBURY LAB,WARRINGTON WA4 4AD,CHESHIRE,ENGLAND
关键词
D O I
10.1088/0953-4075/28/15/015
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The ionization and fragmentation of C and O 1s core excited CO2 has been studied using soft x-rays, threshold electron analysis to define the initial core hole and a triple coincidence technique to examine the final dissociated ion state. The excitation of the O 1s electron results in a single decay channel, CO+ + O+, corresponding to the breaking of a single C-O bond. At the C 1s edge, the same channel is seen together with a weaker channel, corresponding to the triply ionized three-body fragmentation O+ + C+ + O+. Moreover, the angular distribution of ions from the CO+ + O+ channel is seen to depend on the excited-core state.
引用
收藏
页码:3249 / 3260
页数:12
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