BOND-ORBITAL THEORY OF LINEAR AND NONLINEAR ELECTRONIC RESPONSE IN IONIC-CRYSTALS .2. NONLINEAR RESPONSE

被引：95

作者：

LINES, ME

机构：

[1] AT and T Bell Laboratories, Murray Hill

来源：

PHYSICAL REVIEW B | 1990年 / 41卷 / 06期

关键词：

D O I：

10.1103/PhysRevB.41.3383

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

A bond-orbital theory of linear electronic response set out in the preceding companion paper (I) is expanded to include nonlinear response. Attention is focused on the third-order susceptibility ijkl(3) (particularly as measured by the nonlinear refractive index n2) in pretransition-metal halides and chalcogenides. Root-mean-square accuracy over 11 halides for relative n2 values is about 9%, and points to an essential absence of local-field effects in bond-orbital response at least for halides. The latter conclusion enables us to make an absolute calibration for n2a question of some considerable controversy among different experimental groups. © 1990 The American Physical Society.

引用

页码：3383 / 3390

页数：8

共 35 条

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