NEAR-RESONANT SCATTERING FROM NONSYMMETRIC DIMERS - APPLICATIONS TO SUBSTITUTED POLYANILINES

被引:44
作者
LAVARDA, FC [1 ]
DOSSANTOS, MC [1 ]
GALVAO, DS [1 ]
LAKS, B [1 ]
机构
[1] UNESP BAURU,DEPT FIS,BR-17033 BAURU,SP,BRAZIL
关键词
D O I
10.1103/PhysRevLett.73.1267
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
In this work we show that, beyond the prediction of the random dimer model [Wu and Phillips, Phys. Rev. Lett. 66, 1366 (1991)], it is possible to have near resonant scattering from nonsymmetric dimers. It is shown by direct density of states calculations as well as by a procedure similar to the random dimer model that protonated chains of alkyl-substituted polyanilines support extended electronic states at the Fermi energy when a disordered distribution of symmetric or asymmetric bipolarons is present. An extension of the random dimer model to include resonant scattering by nonsymmetric dimers is proposed.
引用
收藏
页码:1267 / 1270
页数:4
相关论文
共 24 条
[11]   ON THE ELECTRONIC-STRUCTURE AND CONDUCTION PROPERTIES OF APERIODIC DNA AND PROTEINS .1. STRATEGY AND METHODS OF INVESTIGATIONS [J].
LADIK, J ;
SEEL, M ;
OTTO, P ;
BAKHSHI, AK .
CHEMICAL PHYSICS, 1986, 108 (02) :203-214
[12]   STABILITY OF POLARONS IN CONDUCTING POLYMERS [J].
MIZES, HA ;
CONWELL, EM .
PHYSICAL REVIEW LETTERS, 1993, 70 (10) :1505-1508
[13]   LOCALIZATION AND ITS ABSENCE - A NEW METALLIC STATE FOR CONDUCTING POLYMERS [J].
PHILLIPS, P ;
WU, HL .
SCIENCE, 1991, 252 (5014) :1805-1812
[14]   ELECTRONIC TRANSPORT AND RESONANCES IN 2 RANDOM DIMER MODELS IN ONE DIMENSION - ANY RELEVANCE TO CONDUCTING POLYANILINE [J].
SEN, AK ;
GANGOPADHYAY, S .
PHYSICA A, 1992, 186 (1-2) :270-284
[15]   EXTENDED STATES IN ONE-DIMENSIONAL LATTICES - APPLICATION TO THE QUASI-PERIODIC COPPER-MEAN CHAIN [J].
SIL, S ;
KARMAKAR, SN ;
MOITRA, RK ;
CHAKRABARTI, A .
PHYSICAL REVIEW B, 1993, 48 (06) :4192-4195
[16]   ELECTRONIC-STRUCTURE OF POLYANILINE AND SUBSTITUTED DERIVATIVES [J].
SNAUWAERT, P ;
LAZZARONI, R ;
RIGA, J ;
VERBIST, JJ .
SYNTHETIC METALS, 1987, 18 (1-3) :335-340
[17]   POLARON LATTICE IN HIGHLY CONDUCTING POLYANILINE - THEORETICAL AND OPTICAL STUDIES [J].
STAFSTROM, S ;
BREDAS, JL ;
EPSTEIN, AJ ;
WOO, HS ;
TANNER, DB ;
HUANG, WS ;
MACDIARMID, AG .
PHYSICAL REVIEW LETTERS, 1987, 59 (13) :1464-1467
[18]  
STREITWIESER A, 1961, MOLECULAR ORBITAL TH, P135
[19]   1ST-PRINCIPLES CALCULATIONS OF THE 3-DIMENSIONAL STRUCTURE AND INTRINSIC DEFECTS IN TRANS-POLYACETYLENE [J].
VOGL, P ;
CAMPBELL, DK .
PHYSICAL REVIEW B, 1990, 41 (18) :12797-12817
[20]   TRANSPORT AND EPR STUDIES OF POLYANILINE - A QUASI-ONE-DIMENSIONAL CONDUCTOR WITH 3-DIMENSIONAL METALLIC STATES [J].
WANG, ZH ;
SCHERR, EM ;
MACDIARMID, AG ;
EPSTEIN, AJ .
PHYSICAL REVIEW B, 1992, 45 (08) :4190-4202