GLOBAL COUPLING IN THE PRESENCE OF DEFECTS - SYNCHRONIZATION IN AN OSCILLATORY SURFACE-REACTION

被引:87
作者
VESER, G
MERTENS, F
MIKHAILOV, AS
IMBIHL, R
机构
[1] Fritz-Haber-Institut der Max-Planck-Gesellschaft, D-14195 Berlin (Dahlem)
关键词
D O I
10.1103/PhysRevLett.71.935
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The transition from a spatially uniformly oscillating surface to the formation of chemical wave patterns has been investigated in the NO+CO reaction on Pt(100) using photoemission electron microscopy. This transition is associated with a discontinuous jump in the local oscillation frequency and can be described as a breakdown of global coupling caused by the presence of defects in the oscillating medium.
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页码:935 / 938
页数:4
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