METHANE EMISSIONS FROM A LANDFILL MEASURED BY EDDY-CORRELATION USING A FAST-RESPONSE DIODE-LASER SENSOR

被引:30
作者
HOVDE, DC [1 ]
STANTON, AC [1 ]
MEYERS, TP [1 ]
MATT, DR [1 ]
机构
[1] NOAA,DIV ATMOSPHER TURBULENCE & DIFFUS,OAK RIDGE,TN 37831
关键词
METHANE; CARBON DIOXIDE; FLUX; LANDFILL; DIODE LASER; EDDY CORRELATION;
D O I
10.1007/BF00696555
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We describe a fast response methane sensor based on the absorption of radiation generated with a near-infrared InGaAsP diode laser. The sensor uses an open path absorption region 0.5 m long; multiple pass optics provide an optical path of 50 m. High frequency wavelength modulation methods give stable signals with detection sensitivity (S/N = 1, 1 Hz bandwidth) for methane of 65 ppb at atmospheric pressure and room temperature. Improvements in the optical stability are expected to lower the current detection limit. We used the new sensor to measure, by eddy correlation, the CH4 flux from a clay-capped sanitary landfill. Simultaneously we measured the Aux of CO2 and H2O. From seven half-hourly periods of data collected after a rainstorm on November 23, 1991, the average flux of CH4 was 17 mmol m(-2) hr(-1) (6400 mg CH4 m(-2) d(-1)) with a coefficient of variation of 25%. This measurement may underrepresent the flux by 15% due to roll-off of the sensor response at high frequency. The landfill was also a source of CO2 with an average flux of 8.1 mmol m(-2) hr(-1) (8550 mg CO2 m(-2) d(-1)) and a coefficient of variation of 26%. A spectral analysis of the data collected from the CH4, CO2, and H2O sensors showed a strong similarity in the turbulent transfer mechanisms.
引用
收藏
页码:141 / 162
页数:22
相关论文
共 52 条
[51]  
WERLE P, 1991, P SOC PHOTO-OPT INS, V1433, P128, DOI 10.1117/12.46159
[52]  
ZAHNISER MS, 1987, AIP C P, V160, P690