COHERENT RADIATIVE CONTROL OF IBR PHOTODISSOCIATION VIA SIMULTANEOUS (OMEGA-1,OMEGA-3) EXCITATION

被引:89
作者
CHAN, CK [1 ]
BRUMER, P [1 ]
SHAPIRO, M [1 ]
机构
[1] WEIZMANN INST SCI,DEPT CHEM PHYS,IL-76100 REHOVOT,ISRAEL
关键词
D O I
10.1063/1.459843
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We show that simultaneous one- and three-photon photodissociation of IBr can be used to control the relative product yield of ground and excited state Br atoms. The control attained is substantial insofar as it is possible to vary the Br* yield over the range of 25%-95%, even for a high J case which involves extensive averaging over M(j) states.
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页码:2688 / 2696
页数:9
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